Two New Fluorogenic Aptasensors Based on Capped Mesoporous Silica Nanoparticles to Detect Ochratoxin A

[EN] Aptamers have been used as recognition elements for several molecules due to their great affinity and selectivity. Additionally, mesoporous nanomaterials have demonstrated great potential in sensing applications. Based on these concepts, we report herein the use of two aptamer¿capped mesoporous...

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Detalles Bibliográficos
Autores: Ribes, Àngela, Santiago Felipe, Sara, Pardo Vicente, María Teresa, Bernardos Bau, Andrea|||0000-0002-3842-5771, Marcos Martínez, María Dolores|||0000-0001-7079-8589, Sancenón Galarza, Félix|||0000-0002-5205-7135, Martínez-Máñez, Ramón|||0000-0001-5873-9674, Aznar, Elena|||0000-0003-0361-3876
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/99372
Acceso en línea:https://riunet.upv.es/handle/10251/99372
Access Level:acceso abierto
Palabra clave:Aptamers
Mesoporous materials
Nanostructures
Ochratoxin A
Sensors
Electron Microscopy Service of the UPV
INGENIERIA DE LA CONSTRUCCION
QUIMICA INORGANICA
QUIMICA ORGANICA
QUIMICA ANALITICA
Descripción
Sumario:[EN] Aptamers have been used as recognition elements for several molecules due to their great affinity and selectivity. Additionally, mesoporous nanomaterials have demonstrated great potential in sensing applications. Based on these concepts, we report herein the use of two aptamer¿capped mesoporous silica materials for the selective detection of ochratoxin¿A (OTA). A specific aptamer for OTA was used to block the pores of rhodamine¿B¿loaded mesoporous silica nanoparticles. Two solids were prepared in which the aptamer capped the porous scaffolds by using a covalent or electrostatic approach. Whereas the prepared materials remained capped in water, dye delivery was selectively observed in the presence of OTA. The protocol showed excellent analytical performance in terms of sensitivity (limit of detection: 0.5¿0.05¿nm), reproducibility, and selectivity. Moreover, the aptasensors were tested for OTA detection in commercial foodstuff matrices, which demonstrated their potential applicability in real samples