N-Iodosuccinimide promoted Hofmann-Löffler Reactions of Sulfonimides under Visible Light

<p> Conditions for an attractive and productive protocol for the position-selective intramolecular C-H amination of aliphatic groups (Hofmann-L&ouml;ffler reaction) are reported employing sulfonimides as nitrogen sources. <em>N</em>-Iodosuccinimide is the only required promoter...

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Detalles Bibliográficos
Autores: O’Broin, Calvin Q., Fernández, Patricia, Martínez, Claudio, Muñiz, Kilian
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/305800
Acceso en línea:http://hdl.handle.net/2072/305800
https://doi.org/10.1021/acs.orglett.5b03476
Access Level:acceso abierto
Descripción
Sumario:<p> Conditions for an attractive and productive protocol for the position-selective intramolecular C-H amination of aliphatic groups (Hofmann-L&ouml;ffler reaction) are reported employing sulfonimides as nitrogen sources. <em>N</em>-Iodosuccinimide is the only required promoter for this transformation, which is conveniently initiated by visible light. The overall transformation provides pyrrolidines under mild and selective conditions as demonstrated for 17 different substrates.</p>