Iridium oxide (IV) nanoparticle-based electrocatalytic detection of PBDE

Polybrominated diphenyl ethers (PBDEs) are a type of flame retardants which are currently banned in EU and USA due their hazardousness for humans and mammals. However, these compounds were highly used during more than 30 years and still persist in the environment since they are resistant to degradat...

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Detalles Bibliográficos
Autores: Quesada-González, Daniel|||0000-0003-3064-2146, Baiocco, Alessandra, Martos, Andrea A., De La Escosura-Muñiz, Alfredo|||0000-0002-9600-0253, Palleschi, Giuseppe, Merkoçi, Arben|||0000-0003-2486-8085
Tipo de recurso: artículo
Fecha de publicación:2019
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:205546
Acceso en línea:https://ddd.uab.cat/record/205546
https://dx.doi.org/urn:doi:10.1016/j.bios.2018.11.050
Access Level:acceso abierto
Palabra clave:Iridium oxide nanoparticles
Flame retardants
PBDEs
Electrocatalysis
Screen printed carbon electrodes
Descripción
Sumario:Polybrominated diphenyl ethers (PBDEs) are a type of flame retardants which are currently banned in EU and USA due their hazardousness for humans and mammals. However, these compounds were highly used during more than 30 years and still persist in the environment since they are resistant to degradation. Herein we present a biosensor for the detection of PBDEs using screen printed carbon electrodes (SPCEs) based on the electrochemical monitoring of water oxidation reaction (WOR) catalyzed by iridium oxide (IV) nanoparticles (IrO NPs). Our assay shows a limit of detection of 21.5 ppb of PBDE in distilled water. We believe that such an IrO NPs-based electrocatalytic sensing system can lead to a rapid, sensitive, low cost and miniaturizable device for the detection of PBDEs.