Microwave-assisted High Diastereoselective Synthesis of (alpha)- Aminophosphonates under Solvent and Catalyst Free-conditions

A simple, efficient and general method has been developed for the high diastereoselective synthesis of a-aminophosphonates through "one-pot" three-component reaction of alkyl and aryl aldehydes with (S)-a-methylbenzylamine or (S)-3,3-dimethyl-2-butylamine and dimethyl phosphite (Kabachnik-...

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Bibliographic Details
Authors: Gaurao D. Tibhe, Miguel Angel Reyes-González, Carlos Cativiela, Mario Ordóñez
Format: article
Status:Published version
Publication Date:2012
Country:México
Institution:Universidad Autónoma del Estado de Morelos
Repository:Redalyc-UAEM
OAI Identifier:oai:redalyc.org:47523306017
Online Access:https://www.redalyc.org/articulo.oa?id=47523306017
Access Level:Open access
Keyword:Química
Three
Microwave
Green Chemistry
aminophosphonates
component Reaction
Description
Summary:A simple, efficient and general method has been developed for the high diastereoselective synthesis of a-aminophosphonates through "one-pot" three-component reaction of alkyl and aryl aldehydes with (S)-a-methylbenzylamine or (S)-3,3-dimethyl-2-butylamine and dimethyl phosphite (Kabachnik-Fields reaction), which proceeds in short time using microwave irradiation under solvent and catalyst free-conditions. This method could be useful in the large-scale synthesis of a-aminophosphonates in short reaction time.