New approaches to the synthesis of pyridinium N-heteroarylaminides

Different substituted pyridinium N-heteroarylaminides have been prepared in one step from N-aminopyridinium iodide and the corresponding heteroaryl halide by two alternative routes. The use of Pd catalysis allowed the easy preparation of products from the less reactive haloheterocycles. The use of w...

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Bibliographic Details
Authors: Córdoba López, Marta, Izquierdo Ceinos, María Luisa, Álvarez-Builla Gómez, Julio
Format: article
Publication Date:2008
Country:España
Institution:Universidad de Alcalá (UAH)
Repository:e_Buah Biblioteca Digital Universidad de Alcalá
Language:English
OAI Identifier:oai:ebuah.uah.es:10017/2691
Online Access:http://hdl.handle.net/10017/2691
https://dx.doi.org/10.1016/j.tet.2008.06.024
Access Level:Open access
Keyword:Palladium-catalyzed amination
Regioselective synthesis
Radical
Cyclization
Suzuki reaction
Aryl bromides
Inner salts
Aminides
Derivatives
N-(2'-azinyl)aminides
N-2'-Pyridylaminide
Chemistry, Organic
Bioquímica
Ciencia
Biochemistry
Science
Description
Summary:Different substituted pyridinium N-heteroarylaminides have been prepared in one step from N-aminopyridinium iodide and the corresponding heteroaryl halide by two alternative routes. The use of Pd catalysis allowed the easy preparation of products from the less reactive haloheterocycles. The use of water as a solvent in conjunction with microwave heating dramatically diminishes the reaction time without having an adverse effect on reaction yields.