Photoredox-Assisted Gold-Catalyzed Arylative Alkoxycyclization of 1,6-Enynes

The photoredox-assisted gold-catalyzed arylative cyclization of 1,6-enynes with aryldiazonium salts gives rise to cyclization products with the opposite configuration at the alkene than that obtained by gold(I)-catalyzed alkoxycyclization. The reaction occurs under mild conditions and shows high fun...

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Bibliographic Details
Authors: Mayans, Joan G., Suppo, Jean-Simon, Echavarren, Antonio M.
Format: article
Status:Versión aceptada para publicación
Publication Date:2020
Country:España
Institution:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repository:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/447789
Online Access:http://hdl.handle.net/2072/447789
https://doi.org/10.1021/acs.orglett.0c00799
Access Level:Open access
Keyword:54
Description
Summary:The photoredox-assisted gold-catalyzed arylative cyclization of 1,6-enynes with aryldiazonium salts gives rise to cyclization products with the opposite configuration at the alkene than that obtained by gold(I)-catalyzed alkoxycyclization. The reaction occurs under mild conditions and shows high functional group tolerance.