Photoredox-Assisted Gold-Catalyzed Arylative Alkoxycyclization of 1,6-Enynes

The photoredox-assisted gold-catalyzed arylative cyclization of 1,6-enynes with aryldiazonium salts gives rise to cyclization products with the opposite configuration at the alkene than that obtained by gold(I)-catalyzed alkoxycyclization. The reaction occurs under mild conditions and shows high fun...

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Detalles Bibliográficos
Autores: Mayans, Joan G., Suppo, Jean-Simon, Echavarren, Antonio M.
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2020
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/447789
Acceso en línea:http://hdl.handle.net/2072/447789
https://doi.org/10.1021/acs.orglett.0c00799
Access Level:acceso abierto
Palabra clave:54
Descripción
Sumario:The photoredox-assisted gold-catalyzed arylative cyclization of 1,6-enynes with aryldiazonium salts gives rise to cyclization products with the opposite configuration at the alkene than that obtained by gold(I)-catalyzed alkoxycyclization. The reaction occurs under mild conditions and shows high functional group tolerance.