Temporal Coherence of Single Photons Emitted by Hexagonal Boron Nitride Defects at Room Temperature

Color centers in hexagonal boron nitride (hBN) emerge as promising quantum light sources at room temperature, with potential applications in quantum communications, among others. The temporal coherence of emitted photons (i.e., their capacity to interfere and distribute photonic entanglement) is ess...

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Detalles Bibliográficos
Autores: Vidal Martínez Pons, Juan Vicente, Kyu Kim, Sang, Behrens, Max, Izquierdo-Molina, Alejandro, Menéndez Rua, Adolfo, Paçal, Serkan, Ateş, Serkan, Viña Liste, Luis M., Antón Solanas, Carlos
Tipo de recurso: artículo
Fecha de publicación:2025
País:España
Institución:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/734060
Acceso en línea:https://hdl.handle.net/10486/734060
https://dx.doi.org/10.1021/acsphotonics.5c02227
Access Level:acceso abierto
Palabra clave:hBN defects
single-photon emitters
quantum optics
temporal coherence
phonon dephasing
michelson interferometry
Física
Descripción
Sumario:Color centers in hexagonal boron nitride (hBN) emerge as promising quantum light sources at room temperature, with potential applications in quantum communications, among others. The temporal coherence of emitted photons (i.e., their capacity to interfere and distribute photonic entanglement) is essential for many of these applications. Hence, it is crucial to study and determine the temporal coherence of this emission under different experimental conditions. In this work, we report the coherence time of the single photons emitted by an hBN defect in a nanocrystal at room temperature, measured via Michelson interferometry. The visibility of this interference vanishes when the temporal delay between the interferometer arms is a few hundred femtoseconds, highlighting that the phonon dephasing processes are 4 orders of magnitude faster than the spontaneous decay time of the emitter. We also analyze the single photon characteristics of the emission via correlation measurements, defect blinking dynamics, and its Debye–Waller factor. Our room temperature results highlight the presence of a strong electron–phonon coupling, suggesting the need to work at cryogenic temperatures to enable quantum photonic applications based on photon interference