High-temperature ferromagnetism in Si:Mn alloys
13 páginas, 3 figuras.-- PACS number(s): 75.50.Pp, 75.50.Cc, 75.75.−c
| Autores: | , , , |
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| Tipo de recurso: | artículo |
| Fecha de publicación: | 2011 |
| País: | España |
| Institución: | Consejo Superior de Investigaciones Científicas (CSIC) |
| Repositorio: | DIGITAL.CSIC. Repositorio Institucional del CSIC |
| OAI Identifier: | oai:digital.csic.es:10261/44082 |
| Acceso en línea: | http://hdl.handle.net/10261/44082 |
| Access Level: | acceso abierto |
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High-temperature ferromagnetism in Si:Mn alloysMen'shov, V. N.Tugushev, V. V.Caprara, S.Chulkov, Eugene V.13 páginas, 3 figuras.-- PACS number(s): 75.50.Pp, 75.50.Cc, 75.75.−cA possible mechanism for high-temperature ferromagnetic order in Si:Mn alloys is proposed. These materials, which are semiconducting or metallic, depending on the Mn content, are suggested to undergo phase separation. In the phase-separated state, again depending on the Mn content, Mn atoms can be gathered within nanometer-sized particles or micrometer-sized islands composed of the MnSi2-z precipitate with z≈(0.25–0.30), which are embedded in the Mn-poor silicon matrix. We consider the MnSi2-z precipitate to be the MnSi1.7 silicide host containing a certain amount of magnetic defects associated with unbound Mn 3d orbitals. The MnSi1.7 silicide is considered to be a weak itinerant ferromagnet, where sizable spin fluctuations (paramagnons) exist far above its intrinsic Curie temperature, leading to a strong enhancement of the exchange coupling between the local moments of the defects. As a result, a significant enhancement of the temperature of onset of long-range order among the local moments may be achieved. We associate this temperature with the global Curie temperature of the precipitate. A phenomenological model is developed to determine the spatial structures and characteristics of ferromagnetic order for the cases of a bulk precipitate and of precipitate particles of various shapes. Moreover, allowing for the presence of strong quenched disorder in the precipitate, we describe short-range ferromagnetic order in the system. Experimental data on Si:Mn alloys are interpreted on the basis of our theoretical results.The work was partially supported by the University of the Basque Country (Proyecto GV UPV/EHU Grant No. IT-366-07), the Spanish Ministerio de Ciencia y Tecnologia (Grant No. FIS2007-66711-C02-01), and the RFBR (Grant No. 10-02-00118). SC also acknowledges financial support by PRIN 2007 under Project No. 2007FW3MJX003. VVT acknowledges financial support by Ikerbasque (Basque Foundation for Science).Peer reviewedAmerican Physical Society201220122011info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501http://hdl.handle.net/10261/44082reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttp://dx.doi.org/10.1103/PhysRevB.83.035201info:eu-repo/semantics/openAccessoai:digital.csic.es:10261/440822026-05-22T06:33:51Z |
| dc.title.none.fl_str_mv |
High-temperature ferromagnetism in Si:Mn alloys |
| title |
High-temperature ferromagnetism in Si:Mn alloys |
| spellingShingle |
High-temperature ferromagnetism in Si:Mn alloys Men'shov, V. N. |
| title_short |
High-temperature ferromagnetism in Si:Mn alloys |
| title_full |
High-temperature ferromagnetism in Si:Mn alloys |
| title_fullStr |
High-temperature ferromagnetism in Si:Mn alloys |
| title_full_unstemmed |
High-temperature ferromagnetism in Si:Mn alloys |
| title_sort |
High-temperature ferromagnetism in Si:Mn alloys |
| dc.creator.none.fl_str_mv |
Men'shov, V. N. Tugushev, V. V. Caprara, S. Chulkov, Eugene V. |
| author |
Men'shov, V. N. |
| author_facet |
Men'shov, V. N. Tugushev, V. V. Caprara, S. Chulkov, Eugene V. |
| author_role |
author |
| author2 |
Tugushev, V. V. Caprara, S. Chulkov, Eugene V. |
| author2_role |
author author author |
| description |
13 páginas, 3 figuras.-- PACS number(s): 75.50.Pp, 75.50.Cc, 75.75.−c |
| publishDate |
2011 |
| dc.date.none.fl_str_mv |
2011 2012 2012 |
| dc.type.none.fl_str_mv |
info:eu-repo/semantics/article http://purl.org/coar/resource_type/c_6501 |
| format |
article |
| dc.identifier.none.fl_str_mv |
http://hdl.handle.net/10261/44082 |
| url |
http://hdl.handle.net/10261/44082 |
| dc.language.none.fl_str_mv |
Inglés |
| language_invalid_str_mv |
Inglés |
| dc.relation.none.fl_str_mv |
http://dx.doi.org/10.1103/PhysRevB.83.035201 |
| dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess |
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openAccess |
| dc.publisher.none.fl_str_mv |
American Physical Society |
| publisher.none.fl_str_mv |
American Physical Society |
| dc.source.none.fl_str_mv |
reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC instname:Consejo Superior de Investigaciones Científicas (CSIC) |
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Consejo Superior de Investigaciones Científicas (CSIC) |
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DIGITAL.CSIC. Repositorio Institucional del CSIC |
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DIGITAL.CSIC. Repositorio Institucional del CSIC |
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1869406993434804224 |
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15.812429 |