Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter

The current transition towards the circular bioeconomy requires a rational development of biorefineries to sustainably fulfill the present demands. The use of Komagataella phaffii (Pichia pastoris) can meet this challenge, since it has the capability to use crude glycerol as a carbon-source, a by-pr...

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Autores: Bernat Camps, Núria, Ebner, Katharina, Schusterbauer, Veronika, Fischer, Jasmin Elgin, Nieto-Taype, Miguel Angel|||0000-0003-1055-0658, Valero, Francisco|||0000-0003-0429-9620, Glieder, Anton|||0000-0002-5986-9689, Garcia-Ortega, Xavier|||0000-0001-7833-3655
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:282622
Acceso en línea:https://ddd.uab.cat/record/282622
https://dx.doi.org/urn:doi:10.3389/fbioe.2023.1130583
Access Level:acceso abierto
Palabra clave:Komagataella phaffii
PDH
Recombinant protein production
Methanol-free expression system
Growth-decoupled bioprocess
Promoter regulation
Pichia pastoris
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spelling Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoterBernat Camps, NúriaEbner, KatharinaSchusterbauer, VeronikaFischer, Jasmin ElginNieto-Taype, Miguel Angel|||0000-0003-1055-0658Valero, Francisco|||0000-0003-0429-9620Glieder, Anton|||0000-0002-5986-9689Garcia-Ortega, Xavier|||0000-0001-7833-3655Komagataella phaffiiPDHRecombinant protein productionMethanol-free expression systemGrowth-decoupled bioprocessPromoter regulationPichia pastorisThe current transition towards the circular bioeconomy requires a rational development of biorefineries to sustainably fulfill the present demands. The use of Komagataella phaffii (Pichia pastoris) can meet this challenge, since it has the capability to use crude glycerol as a carbon-source, a by-product from the biodiesel industry, while producing high- and low-added value products. Recombinant protein production (RPP) using K. phaffii has often been driven either by the methanol induced AOX1 promoter (P) and/or the constitutive GAP promoter (P). In the last years, strong efforts have been focused on developing novel expression systems that expand the toolbox variety of K. phaffii to efficiently produce diverse proteins that requires different strategies. In this work, a study was conducted towards the development of methanol-free expression system based on a heat-shock gene promoter (P) using glycerol as sole carbon source. Using this promoter, the recombinant expression is strongly induced in carbon-starving conditions. The classical P was used as a benchmark, taking for both strains the lipase B from Candida antarctica (CalB) as model protein. Titer of CalB expressed under P outperformed P controlled expression in shake-flask cultivations when using a slow-release continuous feeding technology, confirming that P is induced under pseudo-starving conditions. This increase was also confirmed in fed-batch cultivations. Several optimization rounds were carried out for P under different feeding and osmolarity conditions. In all of them the P controlled process outperformed the P one in regard to CalB titer. The best P approach reached 3.6-fold more specific productivity than P fed-batch at low μ. Compared to the optimum approach for P-based process, the best P fed-batch strategy resulted in 2.3-fold higher titer, while the specific productivity was very similar. To summarize, P is an inducible promoter that exhibited a non-coupled growth regulation showing high performance, which provides a methanol-free additional solution to the usual growth-coupled systems for RPP. Thus, this novel system emerges as a potential alternative for K. phaffii RPP bioprocess and for revaluing crude glycerol, promoting the transition towards a circular economy. 22023-01-0120232023-01-01Articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfhttps://ddd.uab.cat/record/282622https://dx.doi.org/urn:doi:10.3389/fbioe.2023.1130583reponame:Dipòsit Digital de Documents de la UABinstname:Universitat Autònoma de BarcelonaInglésengopen accesshttp://purl.org/coar/access_right/c_abf2Aquest document està subjecte a una llicència d'ús Creative Commons. Es permet la reproducció total o parcial, la distribució, la comunicació pública de l'obra i la creació d'obres derivades, fins i tot amb finalitats comercials, sempre i quan es reconegui l'autoria de l'obra original.https://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:ddd.uab.cat:2826222026-06-06T12:50:31Z
dc.title.none.fl_str_mv Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
title Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
spellingShingle Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
Bernat Camps, Núria
Komagataella phaffii
PDH
Recombinant protein production
Methanol-free expression system
Growth-decoupled bioprocess
Promoter regulation
Pichia pastoris
title_short Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
title_full Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
title_fullStr Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
title_full_unstemmed Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
title_sort Enabling growth-decoupled Komagataella phaffii recombinant protein production based on the methanol-free P promoter
dc.creator.none.fl_str_mv Bernat Camps, Núria
Ebner, Katharina
Schusterbauer, Veronika
Fischer, Jasmin Elgin
Nieto-Taype, Miguel Angel|||0000-0003-1055-0658
Valero, Francisco|||0000-0003-0429-9620
Glieder, Anton|||0000-0002-5986-9689
Garcia-Ortega, Xavier|||0000-0001-7833-3655
author Bernat Camps, Núria
author_facet Bernat Camps, Núria
Ebner, Katharina
Schusterbauer, Veronika
Fischer, Jasmin Elgin
Nieto-Taype, Miguel Angel|||0000-0003-1055-0658
Valero, Francisco|||0000-0003-0429-9620
Glieder, Anton|||0000-0002-5986-9689
Garcia-Ortega, Xavier|||0000-0001-7833-3655
author_role author
author2 Ebner, Katharina
Schusterbauer, Veronika
Fischer, Jasmin Elgin
Nieto-Taype, Miguel Angel|||0000-0003-1055-0658
Valero, Francisco|||0000-0003-0429-9620
Glieder, Anton|||0000-0002-5986-9689
Garcia-Ortega, Xavier|||0000-0001-7833-3655
author2_role author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Komagataella phaffii
PDH
Recombinant protein production
Methanol-free expression system
Growth-decoupled bioprocess
Promoter regulation
Pichia pastoris
topic Komagataella phaffii
PDH
Recombinant protein production
Methanol-free expression system
Growth-decoupled bioprocess
Promoter regulation
Pichia pastoris
description The current transition towards the circular bioeconomy requires a rational development of biorefineries to sustainably fulfill the present demands. The use of Komagataella phaffii (Pichia pastoris) can meet this challenge, since it has the capability to use crude glycerol as a carbon-source, a by-product from the biodiesel industry, while producing high- and low-added value products. Recombinant protein production (RPP) using K. phaffii has often been driven either by the methanol induced AOX1 promoter (P) and/or the constitutive GAP promoter (P). In the last years, strong efforts have been focused on developing novel expression systems that expand the toolbox variety of K. phaffii to efficiently produce diverse proteins that requires different strategies. In this work, a study was conducted towards the development of methanol-free expression system based on a heat-shock gene promoter (P) using glycerol as sole carbon source. Using this promoter, the recombinant expression is strongly induced in carbon-starving conditions. The classical P was used as a benchmark, taking for both strains the lipase B from Candida antarctica (CalB) as model protein. Titer of CalB expressed under P outperformed P controlled expression in shake-flask cultivations when using a slow-release continuous feeding technology, confirming that P is induced under pseudo-starving conditions. This increase was also confirmed in fed-batch cultivations. Several optimization rounds were carried out for P under different feeding and osmolarity conditions. In all of them the P controlled process outperformed the P one in regard to CalB titer. The best P approach reached 3.6-fold more specific productivity than P fed-batch at low μ. Compared to the optimum approach for P-based process, the best P fed-batch strategy resulted in 2.3-fold higher titer, while the specific productivity was very similar. To summarize, P is an inducible promoter that exhibited a non-coupled growth regulation showing high performance, which provides a methanol-free additional solution to the usual growth-coupled systems for RPP. Thus, this novel system emerges as a potential alternative for K. phaffii RPP bioprocess and for revaluing crude glycerol, promoting the transition towards a circular economy.
publishDate 2023
dc.date.none.fl_str_mv 2
2023-01-01
2023
2023-01-01
dc.type.none.fl_str_mv Article
http://purl.org/coar/resource_type/c_6501
VoR
http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://ddd.uab.cat/record/282622
https://dx.doi.org/urn:doi:10.3389/fbioe.2023.1130583
url https://ddd.uab.cat/record/282622
https://dx.doi.org/urn:doi:10.3389/fbioe.2023.1130583
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://creativecommons.org/licenses/by/4.0/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
https://creativecommons.org/licenses/by/4.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:Dipòsit Digital de Documents de la UAB
instname:Universitat Autònoma de Barcelona
instname_str Universitat Autònoma de Barcelona
reponame_str Dipòsit Digital de Documents de la UAB
collection Dipòsit Digital de Documents de la UAB
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