Cerium-doped SrHfO3 sol-gel films

SrHfO3 presents high density, which makes it interesting for host lattice when it is doped with rare earths for luminescent materials. The optical and structural studies of Ce3+-doped strontium hafnate films prepared by the sol-gel process are presented in this work. Crack-free films with waveguidin...

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Detalles Bibliográficos
Autores: Villanueva-Ibáñez,M., Flores-González,M.A., LE Luyer,C.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:Brasil
Institución:Matéria (Rio de Janeiro. Online)
Repositorio:Matéria (Rio de Janeiro. Online)
Idioma:inglés
OAI Identifier:oai:scielo:S1517-70762010000400005
Acceso en línea:http://old.scielo.br/scielo.php?script=sci_arttext&pid=S1517-70762010000400005
Access Level:acceso abierto
Palabra clave:SrHfO3
sol-gel
thin films
planar waveguide
scintillating film
Descripción
Sumario:SrHfO3 presents high density, which makes it interesting for host lattice when it is doped with rare earths for luminescent materials. The optical and structural studies of Ce3+-doped strontium hafnate films prepared by the sol-gel process are presented in this work. Crack-free films with waveguiding performances were obtained with heat-treatments between 400°C and 700°C. The total elimination of organic compounds occurs above 800°C as indicated by Fourier transform infrared spectroscopy. The optogeometric properties (refractive index and thickness) are investigated by m-lines spectroscopy. Films structure is analysed using X-ray diffraction and transmission electron microscopy. The films crystallise from amorphous phase to pure SrHfO3 orthorhombic phase at 750°C. The HfO2 monoclinic phase superposes to SrHfO3 orthorhombic phase after heat treatment performed at 1000°C. Finally, the potentiality to prepare Ce3+ activated SrHfO3 sol-gel films with scintillation properties is explored.