Development of a highly efficient oil degumming process using a novel phosphatidylinositol-specific phospholipase C enzyme

Enzymatic degumming using phospholipase C (PLC) enzymes may be used in environmentally friendly processes with improved oil recovery yields. In this work, phosphatidylinositol-specific phospholipase C (PIPLC) candidates obtained from an in silico analysis were evaluated for oil degumming. A PIPLC fr...

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Bibliographic Details
Authors: Cerminati, Sebastián, Eberhardt, Maria Florencia, Elena, Claudia E., Peirú, Salvador, Castelli, Maria Eugenia, Menzella, Hugo Gabriel
Format: article
Status:Published version
Publication Date:2017
Country:Argentina
Institution:Consejo Nacional de Investigaciones Científicas y Técnicas
Repository:CONICET Digital (CONICET)
Language:English
OAI Identifier:oai:ri.conicet.gov.ar:11336/50530
Online Access:http://hdl.handle.net/11336/50530
Access Level:Open access
Keyword:Enzymatic Degumming
Green Chemistry
Phosphatidylinositol Phospholipase C
Phospholipid Removal
https://purl.org/becyt/ford/2.9
https://purl.org/becyt/ford/2
Description
Summary:Enzymatic degumming using phospholipase C (PLC) enzymes may be used in environmentally friendly processes with improved oil recovery yields. In this work, phosphatidylinositol-specific phospholipase C (PIPLC) candidates obtained from an in silico analysis were evaluated for oil degumming. A PIPLC from Lysinibacillus sphaericus was shown to efficiently remove phosphatidylinositol from crude oil, and when combined with a second phosphatidylcholine and phosphatidylethanolamine-specific phospholipase C, the three major phospholipids were completely hydrolyzed, providing an extra yield of oil greater than 2.1%, compared to standard methods. A remarkably efficient fed-batch Escherichia coli fermentation process producing ∼14 g/L of the recombinant PIPLC enzyme was developed, which may facilitate the adoption of this cost-effective oil-refining process.