Synthesis of self-assembled Ge nanocrystals employing reactive RF sputtering

This work presents the results of a simple methodology able to control crystal size, dispersion and spatial distribution of germanium nanocrystals (Ge-NCs). It takes advantage of a self-assembled process taken place during the deposit of the system SiO$_2$/Ge/SiO$_2$ by reactive RF sputtering. Nanop...

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Detalhes bibliográficos
Autores: Hernández-Hernández, A., Hernández-Hernández, L.A., Marel Monroy, B., Santoyo-Salazar, J., Santana-Rodríguez, G., Márquez-Herrera, A., Gallardo-Hernández, S., Mani-González, P.G., Meléndez-Lira, M.
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2016
País:México
Recursos:UNIVERSIDAD NACIONAL AUTÓNOMA DE MÉXICO
Repositorio:Revista Mexicana de Física
Idioma:inglés
OAI Identifier:oai:ojs2.rmf.smf.mx:article/388
Acesso em linha:https://rmf.smf.mx/ojs/index.php/rmf/article/view/388
Access Level:acceso abierto
Palavra-chave:Nanocrystals
reactive RF sputtering
germanium
heteroestructure
Descrição
Resumo:This work presents the results of a simple methodology able to control crystal size, dispersion and spatial distribution of germanium nanocrystals (Ge-NCs). It takes advantage of a self-assembled process taken place during the deposit of the system SiO$_2$/Ge/SiO$_2$ by reactive RF sputtering. Nanoparticles formation is controlled mainly by the roughness of the first SiO$_2$ layer but the ulterior interaction of the interlayer with the top layer also play a role. Structural quality of germanium nanocrystals increases with roughness and the interlayer thickness. The tetragonal phase of germanium is produced and its crystallographic quality improves with interlayer thickness and oxygen partial pressure. Room temperature photoluminescence emission without a post growth thermal annealing process indicates that our methodology produces a low density of non-radiative traps.