Synthesis, structural characterization and Cu(II) adsorption behavior of manganite (γ-MnOOH) nanorods

"New alternatives for the removal of transition metal ions that present an environmental risk are required. The chemical adsorption of these ions on surfaces with chemisorbent properties represents a promising area of research. In this work, manganite (γ-MnOOH) nanorods were synthesized, with a...

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Detalles Bibliográficos
Autores: LUCIA FABIOLA CANO SALAZAR, ANTONIA MARTINEZ LUEVANOS, JESUS ALEJANDRO CLAUDIO RIZO, FRANCISCO RAUL CARRILLO PEDROZA, SAGRARIO MARTINEZ MONTEMAYOR, JOSE RENE RANGEL MENDEZ
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:México
Institución:Instituto Potosino de Investigación Científica y Tecnológica
Repositorio:Repositorio Institucional del IPICYT
OAI Identifier:oai:ipicyt.repositorioinstitucional.mx:1010/2298
Acceso en línea:http://ipicyt.repositorioinstitucional.mx/jspui/handle/1010/2298
Access Level:acceso abierto
Palabra clave:info:eu-repo/classification/Autor/Aqueous-solution
info:eu-repo/classification/Autor/Copper ions
info:eu-repo/classification/Autor/Removal
info:eu-repo/classification/Autor/Equilibrium
info:eu-repo/classification/Autor/Waste
info:eu-repo/classification/Autor/Hydroxide
info:eu-repo/classification/Autor/Kinetics
info:eu-repo/classification/Autor/Cadmium
info:eu-repo/classification/Autor/Oxides
info:eu-repo/classification/Autor/Zinc
info:eu-repo/classification/cti/2
info:eu-repo/classification/cti/23
Descripción
Sumario:"New alternatives for the removal of transition metal ions that present an environmental risk are required. The chemical adsorption of these ions on surfaces with chemisorbent properties represents a promising area of research. In this work, manganite (γ-MnOOH) nanorods were synthesized, with a surface area of 20.22 m2 g−1, pore size of 32.18 nm and pore volume of 0.1627 cm3 g−1. After chemical and structural characterization of the manganite sample, it was evaluated as an adsorbent of Cu(II) from aqueous solution. The equilibrium adsorption data were well fitted by the Langmuir isotherm, and the results indicated that the maximum adsorption capacity of Cu(II) was 11.926 mg g−1. Cu(II) ion adsorption on the manganite surface is a spontaneous and exothermic process (ΔG°< 0 and ΔH°< 0). The negative value of ΔS° suggests the stability of the adsorption process without structural change at the manganite–aqueous solution interface. A scheme for chemisorption of Cu(II) ions on the hydroxylated surface of manganite is proposed."