Structural Optimization of the Perovskite of Strontium Zirconate: A Study from First Principles

In this work a theoretical study was carried out on the first principles of the structure of strontium zirconate (SrZrO3) type perovskite, which crystallizes in a cubic cell with 5 atoms, specifically 1 Sr atom distributed in the vertices, 3 O atoms in the faces and 1 Zr atom in the center. In the f...

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Detalles Bibliográficos
Autores: Arteaga Varela, Miguel, Herrera Carbajal, Alejandro de Jesús, Reyes Valderrama, María Isabel, Rodriguez Lugo, Ventura
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2019
País:México
Institución:UNIVERSIDAD AUTÓNOMA DEL ESTADO DE HIDALGO
Repositorio:PÄDI Boletín Científico de Ciencias Básicas e Ingeniería del ICBI
Idioma:español
OAI Identifier:oai:repository.uaeh.edu.mx:article/4939
Acceso en línea:https://repository.uaeh.edu.mx/revistas/index.php/icbi/article/view/4939
Access Level:acceso abierto
Palabra clave:Perovskite
Pseudopotential
DFT
Perovskita
Pseudopotencial
Descripción
Sumario:In this work a theoretical study was carried out on the first principles of the structure of strontium zirconate (SrZrO3) type perovskite, which crystallizes in a cubic cell with 5 atoms, specifically 1 Sr atom distributed in the vertices, 3 O atoms in the faces and 1 Zr atom in the center. In the first part of the study, optimization of parameters or an ultra-soft pseudopotential Perdew-Burke-Ernzerhof (PBE) type in Quantum Espresso® code based on Density Functional Theory (DFT). In particular, a series of self-consistent calculations were performed varying the size of the wave function and as the number of high symmetry points in a Monkhorst-Pack grid. Subsequently, a structural optimization was carried out by varying atomic positions and the lattice parameter of the SrZrO3 structure; the band plot and the electronic state density for a Γ, X, R, M, Γ path were obtained. The results obtained show that by means of the lattice parameter that was obtained from simulations of this type of study, structural properties can be obtained with an accuracy of 98.4%.