Cyclic C-F-Metal Containig Species. Solid State and Computational Examples

This article examines the results of research published be- tween 2000 and 2012, which found experimental evidence of cyclic species containing the fragment carbon-fluorine-transition metal. 25 Examples (numbered throughout this paper) with 20 different metals and a wide variety of chemical environm...

Descripción completa

Detalles Bibliográficos
Autores: Maribel Arroyo Carranza, Hugo Torrens Miquel
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2013
País:México
Institución:Universidad Nacional Autónoma de México
Repositorio:Redalyc-UNAM
OAI Identifier:oai:redalyc.org:47527856012
Acceso en línea:https://www.redalyc.org/articulo.oa?id=47527856012
Access Level:acceso abierto
Palabra clave:Química
Carbon
theory
fluorine
structure
bond activation
Descripción
Sumario:This article examines the results of research published be- tween 2000 and 2012, which found experimental evidence of cyclic species containing the fragment carbon-fluorine-transition metal. 25 Examples (numbered throughout this paper) with 20 different metals and a wide variety of chemical environments have been gathered. A similar analysis brings together almost 40 transitional states and intermediates resulting from theoretical work studying the transition metal mediated carbon-fluorine bond activation. Among other aspects, this review is useful to recognize the specific characteristics which determine whether the C-F activation process is carried out through a concerted process, a mechanism assisted by auxiliary ligands or by free radicals.