Dual Co/Photoredox-Catalyzed Regio- and Stereoselective Synthesis of Highly Functional 1,3-Dienes

A dual Co/photoredox catalytic coupling of 1,3-enynes and α,ß-unsaturated aliphatic aldehydes and ketones has been developed that creates access to highly functional 1,3-diene synthons through a regio- and stereoselective carbon-carbon coupling process. The scope of the process features diverse func...

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Detalles Bibliográficos
Autores: Tóth, Balázs L., Delgado, Alejandro, Ghorai, Debasish, Meneses, Diego, García-Camacho, Aimara, Vicent-Morales, Maria, Benet-Buchholz, Jordi, Funes-Ardoiz, Ignacio, Kleij, Arjan W.
Tipo de recurso: artículo
Fecha de publicación:2025
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/489064
Acceso en línea:http://hdl.handle.net/2072/489064
https://doi.org/10.1002/anie.202522561
Access Level:acceso embargado
Palabra clave:Química
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Descripción
Sumario:A dual Co/photoredox catalytic coupling of 1,3-enynes and α,ß-unsaturated aliphatic aldehydes and ketones has been developed that creates access to highly functional 1,3-diene synthons through a regio- and stereoselective carbon-carbon coupling process. The scope of the process features diverse functionalized scaffolds with a high degree of molecular complexity. The synthetic utility of these 1,3-dienes is demonstrated including a telescoped, one-pot approach using an alkynyl cyclic carbonate as a 1,3-enyne surrogate offering direct access to the 1,3-diene product. Mechanistic analysis involving control reactions, deuterium labeling studies and DFT calculations are in line with the in situ formation of a Co─H species and an outer-sphere coupling pathway in which a regio- and stereoselective coupling occurs between a dienyl radical and carbonyl species.