Influence of oxygen plasma treatment parameters on poly(vinylidene fluoride) electrospun fiber mats wettability

[EN] Electrospun poly(vinylidene fluoride) (PVDF) fiber mats find applications in an increasing number of areas, such as battery separators, filtration and detection membranes, due to their excellent properties. However, there are limitations due to the hydrophobic nature and low surface energy of P...

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Detalles Bibliográficos
Autores: Correia, Daniela M., Ribeiro, Clarisse, Sencadas, Vitor Joao Gomes Da Silva, Botelho, G., Carabineiro, S.A.C., Lanceros-Mendez, Senentxu, Gómez Ribelles, José Luís|||0000-0001-9099-0885
Tipo de recurso: artículo
Fecha de publicación:2015
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/71307
Acceso en línea:https://riunet.upv.es/handle/10251/71307
Access Level:acceso abierto
Palabra clave:Electrospun membranes
Electroactive PVDF
Oxygen plasma treatment
Surface modification
Surface wettability
Oxidation mechanism
MAQUINAS Y MOTORES TERMICOS
Descripción
Sumario:[EN] Electrospun poly(vinylidene fluoride) (PVDF) fiber mats find applications in an increasing number of areas, such as battery separators, filtration and detection membranes, due to their excellent properties. However, there are limitations due to the hydrophobic nature and low surface energy of PVDF. In this work, oxygen plasma treatment has been applied in order to modify the surface wettability of PVDF fiber mats and superhydrophilic PVDF electrospun membranes have been obtained. Further, plasma treatment does not significantly influences fiber average size (similar to 400 +/- 200 nm), morphology, electroacfive beta-phase content (similar to 80-85%) or the degree of crystallinity (X-c of 42 +/- 2%), allowing to maintain the excellent physical-chemical characteristics of PVDF. Plasma treatment mainly induces surface chemistry modifications, such as the introduction of oxygen and release of fluorine atoms that significantly changes polymer membrane wettability by a reduction of the contact angle of the polymer fibers and an overall decrease of the surface tension of the membranes.