Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion

Video S1, the motion of bare α-Fe2O3 nanorod under dark and blue light illumination in 0.1% H2O2

Detalles Bibliográficos
Autores: Chen, Yufen, Li, Chunyu, Ferrer Campos, Rebeca, Esplandiú, María J., Fraxedas, J., Liguori, Nicoletta, Villa, Katherine
Tipo de recurso: conjunto de datos
Fecha de publicación:2025
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/398519
Acceso en línea:http://hdl.handle.net/10261/398519
Access Level:acceso abierto
Palabra clave:Transient absorption spectroscopy
Ray photoelectron spectroscopy
Engineering semiconductor heterostructures
Efficient electron mediator
Ambient pressure x
Pt significantly enhances
Pt layer exhibit
Intermediate pt layer
Promote charge separation
Responsive nanomotor based
Unraveling charge transport
Charge transport
Pt serves
Based near
Trilayered heterostructure
Targeted delivery
Synchrotron radiation
Significant efforts
Rational strategy
Promising tools
Modest propulsion
Environmental remediation
Driven propulsion
Combining narrow
Clear understanding
Bandgap α
Advanced techniques
id ES_fa38e97d47247cfce0265d7cd154d924
oai_identifier_str oai:digital.csic.es:10261/398519
network_acronym_str ES
network_name_str España
repository_id_str
spelling Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic MotionChen, YufenLi, ChunyuFerrer Campos, RebecaEsplandiú, María J.Fraxedas, J.Liguori, NicolettaVilla, KatherineTransient absorption spectroscopyRay photoelectron spectroscopyEngineering semiconductor heterostructuresEfficient electron mediatorAmbient pressure xPt significantly enhancesPt layer exhibitIntermediate pt layerPromote charge separationResponsive nanomotor basedUnraveling charge transportCharge transportPt servesBased nearTrilayered heterostructureTargeted deliverySynchrotron radiationSignificant effortsRational strategyPromising toolsModest propulsionEnvironmental remediationDriven propulsionCombining narrowClear understandingBandgap αAdvanced techniquesVideo S1, the motion of bare α-Fe2O3 nanorod under dark and blue light illumination in 0.1% H2O2Photocatalytic micro/nanomotors have emerged as promising tools for environmental remediation, biosensing, and targeted delivery. To enhance their light-driven propulsion, significant efforts have focused on engineering semiconductor heterostructures, which promote charge separation. However, a clear understanding of how these architectures govern photocatalytic mechanisms and influence motion performance remains limited. Here, we design a visible light-responsive nanomotor based on a Fe2O3-Pt-TiO2 trilayered heterostructure, combining narrow-bandgap α-Fe2O3 and wide-bandgap TiO2 with an intermediate Pt layer. Remarkably, Fe2O3-TiO2 nanomotors without the Pt layer exhibit only modest propulsion under visible light, whereas the inclusion of Pt significantly enhances their motility. Through advanced techniques, including in situ synchrotron radiation-based near-ambient pressure X-ray photoelectron spectroscopy and transient absorption spectroscopy, we reveal that Pt serves as an efficient electron mediator, enabling directional charge transfer across the heterojunction. This study provides fundamental insights into charge transport in multicomponent nanomotors and introduces a rational strategy for designing efficient photoactive systems.Peer reviewedFigshareFraxedas, J. [0000-0002-2821-4831]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202520252025info:eu-repo/semantics/datasethttp://purl.org/coar/resource_type/c_ddb1video/mp4http://hdl.handle.net/10261/398519reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)InglésChen, Yufen; Li, Chunyu; Ferrer Campos, Rebeca; Esplandiú, María J.; Fraxedas, J.; Liguori, Nicoletta; Villa, Katherine. Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion. https://doi.org/10.1021/acs.nanolett.5c02177. http://hdl.handle.net/10261/398057https://doi.org/10.1021/acs.nanolett.5c02177.s002Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3985192026-05-22T06:33:51Z
dc.title.none.fl_str_mv Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
title Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
spellingShingle Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
Chen, Yufen
Transient absorption spectroscopy
Ray photoelectron spectroscopy
Engineering semiconductor heterostructures
Efficient electron mediator
Ambient pressure x
Pt significantly enhances
Pt layer exhibit
Intermediate pt layer
Promote charge separation
Responsive nanomotor based
Unraveling charge transport
Charge transport
Pt serves
Based near
Trilayered heterostructure
Targeted delivery
Synchrotron radiation
Significant efforts
Rational strategy
Promising tools
Modest propulsion
Environmental remediation
Driven propulsion
Combining narrow
Clear understanding
Bandgap α
Advanced techniques
title_short Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
title_full Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
title_fullStr Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
title_full_unstemmed Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
title_sort Video S1: Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion
dc.creator.none.fl_str_mv Chen, Yufen
Li, Chunyu
Ferrer Campos, Rebeca
Esplandiú, María J.
Fraxedas, J.
Liguori, Nicoletta
Villa, Katherine
author Chen, Yufen
author_facet Chen, Yufen
Li, Chunyu
Ferrer Campos, Rebeca
Esplandiú, María J.
Fraxedas, J.
Liguori, Nicoletta
Villa, Katherine
author_role author
author2 Li, Chunyu
Ferrer Campos, Rebeca
Esplandiú, María J.
Fraxedas, J.
Liguori, Nicoletta
Villa, Katherine
author2_role author
author
author
author
author
author
dc.contributor.none.fl_str_mv Fraxedas, J. [0000-0002-2821-4831]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Transient absorption spectroscopy
Ray photoelectron spectroscopy
Engineering semiconductor heterostructures
Efficient electron mediator
Ambient pressure x
Pt significantly enhances
Pt layer exhibit
Intermediate pt layer
Promote charge separation
Responsive nanomotor based
Unraveling charge transport
Charge transport
Pt serves
Based near
Trilayered heterostructure
Targeted delivery
Synchrotron radiation
Significant efforts
Rational strategy
Promising tools
Modest propulsion
Environmental remediation
Driven propulsion
Combining narrow
Clear understanding
Bandgap α
Advanced techniques
topic Transient absorption spectroscopy
Ray photoelectron spectroscopy
Engineering semiconductor heterostructures
Efficient electron mediator
Ambient pressure x
Pt significantly enhances
Pt layer exhibit
Intermediate pt layer
Promote charge separation
Responsive nanomotor based
Unraveling charge transport
Charge transport
Pt serves
Based near
Trilayered heterostructure
Targeted delivery
Synchrotron radiation
Significant efforts
Rational strategy
Promising tools
Modest propulsion
Environmental remediation
Driven propulsion
Combining narrow
Clear understanding
Bandgap α
Advanced techniques
description Video S1, the motion of bare α-Fe2O3 nanorod under dark and blue light illumination in 0.1% H2O2
publishDate 2025
dc.date.none.fl_str_mv 2025
2025
2025
dc.type.none.fl_str_mv info:eu-repo/semantics/dataset
http://purl.org/coar/resource_type/c_ddb1
format dataset
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/398519
url http://hdl.handle.net/10261/398519
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv Chen, Yufen; Li, Chunyu; Ferrer Campos, Rebeca; Esplandiú, María J.; Fraxedas, J.; Liguori, Nicoletta; Villa, Katherine. Unraveling Charge Transport in Heterostructured Nanomotors for Efficient Photocatalytic Motion. https://doi.org/10.1021/acs.nanolett.5c02177. http://hdl.handle.net/10261/398057
https://doi.org/10.1021/acs.nanolett.5c02177.s002
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv video/mp4
dc.publisher.none.fl_str_mv Figshare
publisher.none.fl_str_mv Figshare
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869425164881494016
score 15,812429

Similares en LA Referencia