Competing charge ordering and Mott phases in a correlated Sn/Ge(111) two-dimensional triangular lattice

We take advantage of complementary high-resolution experimental techniques and theoretical tools to get insight into the alpha-Sn/Ge(111) triangular lattice surface consisting of sp electrons. We report a (3 x 3) phase, characterized by a charge ordering settled by electronic correlation, which appe...

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Detalles Bibliográficos
Autores: Cortés, R, Tejeda, A., Lobo Checa, J., Didiot, C., Kierren, B., Malterre, D., Merino, J., Flores, F., Michel, E. G., Mascaraque Susunaga, Arantzazu
Tipo de recurso: artículo
Fecha de publicación:2013
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/33766
Acceso en línea:https://hdl.handle.net/20.500.14352/33766
Access Level:acceso abierto
Palabra clave:538.9
Surface phase
Transition
Temperature
Pb/Ge(111)
Systems
Sn/Ge(Iii)
Insulator
Defects
Phonon
State
Física de materiales
Descripción
Sumario:We take advantage of complementary high-resolution experimental techniques and theoretical tools to get insight into the alpha-Sn/Ge(111) triangular lattice surface consisting of sp electrons. We report a (3 x 3) phase, characterized by a charge ordering settled by electronic correlation, which appears between the known metallic-(3 x 3) and Mott insulator phases. We identify the atomistic mechanism behind the stabilization of this phase and interpret these findings on the basis of theoretical calculations. We disentangle the role of the various degrees of freedom in the stability of the different phases found and describe the stepwise surface changes between the metallic and Mott insulating phases.