Solution-phase synthesis and photoluminescence of quaternary chalcohalide semiconductors

Mixed-metal chalcohalide semiconductors have emerged as promising candidates for photovoltaic applications. However, preparation of these multinary compounds using solution-phase techniques remains particularly challenging compared to traditional solid-state methods. To fully harness their potential...

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Detalles Bibliográficos
Autores: Roth, Alison N., Opare-Addo, Jemima, Gi, Eunbyeol|||0000-0003-0846-8655, Mena Fernández, Silvia|||0000-0002-2800-2388, Guirado, Gonzalo|||0000-0003-2128-7007, Schaller, Richard D.|||0000-0001-9696-8830, Smith, Emily A.|||0000-0001-7438-7808, Vela, Javier|||0000-0001-5124-6893
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:274565
Acceso en línea:https://ddd.uab.cat/record/274565
https://dx.doi.org/urn:doi:10.1021/acs.chemmater.3c00011
Access Level:acceso abierto
Palabra clave:Chalcohalides
Quaternary semiconductors
Solution synthesis
Photoluminescence
Fine tuning
Mixed-metals
Phase purity
Photovoltaic applications
Reaction parameters
Rod-like morphology
Solid state method
Solution phase
Solution phase synthesis
Synthetic methods
Descripción
Sumario:Mixed-metal chalcohalide semiconductors have emerged as promising candidates for photovoltaic applications. However, preparation of these multinary compounds using solution-phase techniques remains particularly challenging compared to traditional solid-state methods. To fully harness their potential, it is desirable to develop synthetic methods that enable control over both the phase purity and dimensionality of chalcohalides. Here, we report the solution-phase synthesis of PbSbSI and PbBiSI quaternary chalcohalides using readily available precursors. Fine tuning of reaction parameters allows for the isolation of rod-like morphologies with tunable diameters and aspect ratios. The quaternary chalcohalides display photoluminescence as an ensemble as well as at the single particle level, as demonstrated using fluorescence microscopy. We further evaluate the relative stability and band gap of PbSbSI polymorphs and their coloring patterns using electronic structure calculations. The synthetic methods developed here will motivate the study of ever more complex chalcohalides and other multinary semiconductors for new technological applications.