Properties of Nanocrystalline Silicon Probed by Optomechanics

Nanocrystalline materials exhibit properties that can differ substantially from those of their single crystal counterparts. As such, they provide ways to enhance and optimize their functionality for devices and applications. Here, we report on the optical, mechanical and thermal properties of nanocr...

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Detalhes bibliográficos
Autores: Navarro Urrios, Daniel, Colombano, Martín F., Maire, Jérémie, Chavez Ángel, Emigdio, Arregui, Guillermo, Capuj, Néstor E., Devos, Arnaud, Griol, Amadeu, Bellieres, Laurent, Martínez, Alejandro, Grigoras, Kestutis, Häkkinen, Teija, Saarilahti, Jaakko, Makkonen, Tapani, Sotomayor Torres, Clivia M., Ahopelto, Jouni
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2020
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositório:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/179458
Acesso em linha:https://hdl.handle.net/2445/179458
Access Level:Acceso aberto
Palavra-chave:Ones electromagnètiques
Silici
Electromagnetic waves
Silicon
Descrição
Resumo:Nanocrystalline materials exhibit properties that can differ substantially from those of their single crystal counterparts. As such, they provide ways to enhance and optimize their functionality for devices and applications. Here, we report on the optical, mechanical and thermal properties of nanocrystalline silicon probed by means of optomechanical nanobeams to extract information of the dynamics of optical absorption, mechanical losses, heat generation and dissipation. The optomechanical nanobeams are fabricated using nanocrystalline films prepared by annealing amorphous silicon layers at different temperatures. The resulting crystallite sizes and the stress in the films can be controlled by the annealing temperature and time and, consequently, the properties of the films can be tuned relatively freely, as demonstrated here by means of electron microscopy and Raman scattering. We show that the nanocrystallite size and the volume fraction of the grain boundaries play a key role in the dissipation rates through nonlinear optical and thermal processes. Promising optical (13,000) and mechanical (1700) quality factors were found in the optomechanical cavity realized in the nanocrystalline Si resulting from annealing at 950°C. The enhanced absorption and recombination rates via the intragap states and the reduced thermal conductivity boost the potential to exploit these nonlinear effects in applications including Nanoelectromechanical systems (NEMS), phonon lasing and chaos-based devices.