Synthesis of mono‑n‑methyl aromatic amines from nitroso compounds and methylboronic acid

The selective synthesis of mono-N-methyl aromatic amines was achieved by the reaction of aromatic nitroso compounds with methylboronic acid promoted by triethylphosphite under transition metal-free conditions. The target compounds are constructed efficiently without overmethylation, under environmen...

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Detalles Bibliográficos
Autores: García Csaky, Aurelio, Roscales García, Silvia
Tipo de recurso: artículo
Fecha de publicación:2019
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/113025
Acceso en línea:https://hdl.handle.net/20.500.14352/113025
Access Level:acceso abierto
Palabra clave:547
Boronic acids
Amination reaction
Nitroso compounds
Química orgánica (Química)
2306 Química Orgánica
Descripción
Sumario:The selective synthesis of mono-N-methyl aromatic amines was achieved by the reaction of aromatic nitroso compounds with methylboronic acid promoted by triethylphosphite under transition metal-free conditions. The target compounds are constructed efficiently without overmethylation, under environmentally benign reaction conditions that do not require bases or reductants and therefore are of interest in pharmaceutical, agricultural, and chemical industries.