Synthesis of Novel 3-Amino(Hydroxy)methyl-l-fuco-Azafagomines as Leads for Selective Inhibitors of α-l-Fucosidases

The synthesis of 3-substituted l-fuco-azafagomines from d-lyxose is reported. They represent the first example of aza-C-glycosides having a biimino (-NH-NH-) moiety. The key step of the synthesis is the introduction of the hydrazine moiety by reductive hydrazination of a 1-deoxy-ketohexose with tert...

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Detalles Bibliográficos
Autores: Moreno Clavijo, Elena, Carmona Asenjo, Ana Teresa, Moreno Vargas, Antonio José, Álvarez González, Eleuterio, Robina Ramírez, Inmaculada
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/70186
Acceso en línea:https://hdl.handle.net/11441/70186
https://doi.org/10.1055/s-0029-1219906
Access Level:acceso abierto
Palabra clave:Azasugars
Glycosidases
Fucosidase inhibitors
Aza-fagomines
C-glycosides
Descripción
Sumario:The synthesis of 3-substituted l-fuco-azafagomines from d-lyxose is reported. They represent the first example of aza-C-glycosides having a biimino (-NH-NH-) moiety. The key step of the synthesis is the introduction of the hydrazine moiety by reductive hydrazination of a 1-deoxy-ketohexose with tert-butyl carbazate. Their glycosidase inhibitory properties are also reported.