Emergence of large spin-charge interconversion at an oxidized Cu/W interface

Spin-orbitronic devices can integrate memory and logic by exploiting spin-charge interconversion (SCI), which is optimized by design and materials selection. In these devices, interfaces are crucial elements as they can prohibit or promote spin flow in a device as well as possess spin-orbit coupling...

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Detalles Bibliográficos
Autores: Groen, Inge, Pham, Van Tuong, Ilić, Stefan, Chuvilin, Andrey, Choi, Won Young, Sagasta, Edurne, Vaz, Diogo C., Arango, Isabel C., Ontoso, Nerea, Bergeret, F. Sebastian, Hueso, Luis E., Tokatly, Ilya, Casanova, Félix
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2023
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:dnet:digitalcsic_::39aa08116f1a505a1a3626067ebaa8d9
Acceso en línea:http://hdl.handle.net/10261/342295
Access Level:acceso abierto
Descripción
Sumario:Spin-orbitronic devices can integrate memory and logic by exploiting spin-charge interconversion (SCI), which is optimized by design and materials selection. In these devices, interfaces are crucial elements as they can prohibit or promote spin flow in a device as well as possess spin-orbit coupling resulting in interfacial SCI. Therefore, investigation of interfaces in spin-orbitronic devices is important. Here, we study the origin of SCI in a Py/Cu/W lateral spin valve and quantify its efficiency. An exhaustive characterization of the interface between Cu and W electrodes uncovers the presence of an oxidized layer (WOx). We determine that the SCI occurs at the Cu/WOx interface with a temperature-independent interfacial spin-loss conductance of G∥≈20×1013Ω−1m−2 and an interfacial spin-charge conductivity σSC=−1600Ω−1cm−1 at 10 K (−800Ω−1cm−1 at 300 K). This corresponds to an efficiency given by the inverse Edelstein length λIEE=− 0.8nm at 10 K (−0.4nm at 300 K), which is remarkably larger than in metal/metal and metal/oxide interfaces and bulk heavy metals. The large SCI efficiency at such an oxidized interface makes it a promising candidate for the magnetic readout in MESO logic devices.