Metabolically Active, Fully Hydrolysable Polymersomes

The synthesis and aqueous self-assembly of a new class of amphiphilic aliphatic polyesters are presented. These AB block polyesters comprise polycaprolactone (hydrophobe) and an alternating polyester from succinic acid and an ether-substituted epoxide (hydrophile). They self-assemble into biodegrada...

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Detalles Bibliográficos
Autores: Zhu, Yunqing, Poma, Alessandro, Rizzello, Loris, Gouveia, Virginia M., Ruiz‐Perez, Lorena, Battaglia, Giuseppe, Williams, Charlotte K.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2019
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/216542
Acceso en línea:https://hdl.handle.net/2445/216542
Access Level:acceso abierto
Palabra clave:Agents tensioactius
Polièsters
Química
Surface active agents
Polyesters
Chemistry
Descripción
Sumario:The synthesis and aqueous self-assembly of a new class of amphiphilic aliphatic polyesters are presented. These AB block polyesters comprise polycaprolactone (hydrophobe) and an alternating polyester from succinic acid and an ether-substituted epoxide (hydrophile). They self-assemble into biodegradable polymersomes capable of entering cells. Their degradation products are bioactive, giving rise to differentiated cellular responses inducing stromal cell proliferation and macrophage apoptosis. Both effects emerge only when the copolymers enter cells as polymersomes and their magnitudes are size dependent.