Terahertz spin-light coupling in proximitized Dirac materials

The two-dimensional (2D) materials are highly susceptible to the influence of their neighbors, thereby enabling the design by proximity phenomena. We reveal a remarkable terahertz (THz) spin-light interaction in 2D Dirac materials that arises from magnetic and spin-orbital proximity effects. The dyn...

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Detalles Bibliográficos
Autores: Denisov, Konstantin S.|||0000-0002-1477-3667, Rozhansky, Igor V.|||0000-0001-9391-9304, Valenzuela, Sergio O.|||0000-0002-4632-8891, Žutić, Igor|||0000-0003-2485-226X
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:308320
Acceso en línea:https://ddd.uab.cat/record/308320
https://dx.doi.org/urn:doi:10.1103/PhysRevB.109.L201406
Access Level:acceso abierto
Palabra clave:Dirac electrons
Electric dipole spin resonance
Light couplings
Light interaction
Magnetic orbitals
Proximity effects
Pseudospin
Spin-orbitals
Tera Hertz
Two-dimensional
Descripción
Sumario:The two-dimensional (2D) materials are highly susceptible to the influence of their neighbors, thereby enabling the design by proximity phenomena. We reveal a remarkable terahertz (THz) spin-light interaction in 2D Dirac materials that arises from magnetic and spin-orbital proximity effects. The dynamical realization of the spin-charge conversion, the electric dipole spin resonance (EDSR), of Dirac electrons displays distinctive THz features upon emerging spin-pseudospin proximity terms in the Hamiltonian. To capture the effect of fast pseudospin dynamics on the electron spin, we develop a mean-field theory and complement it with a quantum-mechanical treatment. As a specific example, we investigate the THz response of a single graphene layer proximitized by a magnetic substrate. Our analysis demonstrates a strong enhancement and anomalous polarization structure of the THz-light absorption, which can enable THz detection and efficient generation and control of spins in spin-based quantum devices. The identified coupled spin-pseudospin dynamics is not limited to EDSR and may influence a broad range of optical, transport, and ultrafast phenomena.