Few-layer antimonene electrical properties

Antimonene -a single layer of antimony atoms- and its few layer forms are among the latest additions to the 2D mono-elemental materials family. Numerous predictions and experimental evidence of its remarkable properties including (opto)electronic, energetic or biomedical, among others, together with...

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Detalhes bibliográficos
Autores: Ares García, Pablo, Pakdel, Sahar, Palacio, Irene, Paz, Wendel S., Rassekh, Maedeh, Rodríguez-San Miguel, David, Aballe, Lucía, Foerster, Michael, Ruiz del Árbol, Nerea, Martín-Gago, José Ángel, Zamora Abanades, Félix Juan, Gómez Herrero, Julio, Palacios Burgos, Juan José
Tipo de documento: artigo
Data de publicação:2021
País:España
Recursos:Universidad Autónoma de Madrid
Repositório:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglês
OAI Identifier:oai:repositorio.uam.es:10486/700480
Acesso em linha:http://hdl.handle.net/10486/700480
https://dx.doi.org/10.1016/j.apmt.2021.101132
Access Level:Acceso aberto
Palavra-chave:Antimony atoms
Photoemission electron microscopy
Kelvin probe force microscopy
Electronic properties
Física
Descrição
Resumo:Antimonene -a single layer of antimony atoms- and its few layer forms are among the latest additions to the 2D mono-elemental materials family. Numerous predictions and experimental evidence of its remarkable properties including (opto)electronic, energetic or biomedical, among others, together with its robustness under ambient conditions, have attracted the attention of the scientific community. However, experimental evidence of its electrical properties is still lacking. Here, we characterized the electronic properties of mechanically exfoliated flakes of few-layer (FL) antimonene of different thicknesses (∼ 2–40 nm) through photoemission electron microscopy, kelvin probe force microscopy and transport measurements, which allows us to estimate a sheet resistance of ∼ 1200 Ω sq−1 and a mobility of ∼ 150 cm2V−1s−1 in ambient conditions, independent of the flake thickness. Alternatively, our theoretical calculations indicate that topologically protected surface states (TPSS) should play a key role in the electronic properties of FL antimonene, which supports our experimental findings. We anticipate our work will trigger further experimental studies on TPSS in FL antimonene thanks to its simple structure and significant stability in ambient environments