Unlocking the Potential of Different Types of Biomass- Derived Carbon Dots as Fluorescence Lifetime Imaging Probes

The ongoing search for innovative and environmentally friendly luminescent materials coupled with customizable physical and chemical properties at the nanoscale positions carbon dots (CDots) as ideal candidates for photonic applications. However, even today, their rational design for specific applic...

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Detalles Bibliográficos
Autores: Rosell de la Fuente, María, Torregrosa Rivero, Verónica, Herrera Ochoa, Diego, Garzón Ruiz, Andrés, García Martínez, Javier, Serrano, Elena, Martín Álvarez, Cristina
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universidad de Castilla-La Mancha
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/41567
Acceso en línea:https://doi.org/10.1002/cptc.202400133
https://hdl.handle.net/10578/41567
Access Level:acceso abierto
Palabra clave:Carbon dots
Descripción
Sumario:The ongoing search for innovative and environmentally friendly luminescent materials coupled with customizable physical and chemical properties at the nanoscale positions carbon dots (CDots) as ideal candidates for photonic applications. However, even today, their rational design for specific applications remains elusive due to the unknown relationship between optical and structural properties. Therefore, this study aims to fill this gap by linking the chemical structure of the precursor and synthetic conditions to the final structural composition of the CDots and, by extension, to their optical properties. The study shows that while CDots are chemically stable, their optical properties, which are determined by the carbonaceous core and surface groups, are highly pH dependent. These properties, together with the long fluorescence lifetimes observed in living cells (>10 ns), make these biomass-derived CDots promising probes for time-resolved fluorescence imaging.