Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers

Anomalous Nernst (ANE) and spin Seebeck effects (SSE) are ubiquitous in conducting magnetic materials subject to temperature gradients. Their characterization in metallic systems is especially strenuous because of their indistinguishable symmetry. Here, we report on the accurate characterization of...

Descripción completa

Detalles Bibliográficos
Autores: Sousa, J. Alejandro de, Damerio, Silvia, Koraltan, Sabri, Avci, Can Onur
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2025
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/385274
Acceso en línea:http://hdl.handle.net/10261/385274
https://api.elsevier.com/content/abstract/scopus_id/85216888579
Access Level:acceso abierto
Palabra clave:Metrology
Nernst effect
Spin Seebeck effect
Spin caloritronics
Transport phenomena
Heterostructures
Magnetic multilayers
Transition metals
id ES_bc348e52cbc4e4f0636b959f7b560c6c
oai_identifier_str oai:digital.csic.es:10261/385274
network_acronym_str ES
network_name_str España
repository_id_str
spelling Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayersSousa, J. Alejandro deDamerio, SilviaKoraltan, SabriAvci, Can OnurMetrologyNernst effectSpin Seebeck effectSpin caloritronicsTransport phenomenaHeterostructuresMagnetic multilayersTransition metalsAnomalous Nernst (ANE) and spin Seebeck effects (SSE) are ubiquitous in conducting magnetic materials subject to temperature gradients. Their characterization in metallic systems is especially strenuous because of their indistinguishable symmetry. Here, we report on the accurate characterization of the ANE and SSE in Fe-based multilayers at and above room temperature. We reveal that both effects consist of temperature-dependent and -independent components. At high temperatures, we provide evidence that the ANE decreases mainly due to reduced magnetization and spin polarization of free electrons, whereas the SSE increases owing to the enhanced thermal magnon density. We show that the relative strength of ANE and SSE can be tuned by thickness, stacking order, and doping concentration in various Fe-based multilayers, opening the way for thermoelectric device engineering.We thank Stefano Fedel and Matteo Fettizio for insightful discussions. J.A.D.S. and C.O.A. acknowledge funding from the CONVERT project with administrative reference TED2021-129540A-I00 financed by MCIN/AEI/10.13039/501100011033 and the European Union through the “NextGenerationEU” funds. C.O.A. acknowledges funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (project MAGNEPIC, Grant Agreement No. 949052). S.D. acknowledges funding from the Marie Skłodowska-Curie Actions (MSCA) under the European Union’s Horizon Europe research and innovation programme (project SPINDY, Grant Agreement No. 101106885). J.A.D.S., C.O.A., and S.D. acknowledge financial support from the State Investigation Agency, through the Severo Ochoa Programme for Centres of Excellence in R&D (CEX2023-001263-S).With funding from the Spanish government through the ‘Severo Ochoa Centre of Excellence’ accreditation (CEX2023-001263-S).Peer reviewedAmerican Physical SocietyMinisterio de Ciencia e Innovación (España)European CommissionEuropean Research CouncilAgencia Estatal de Investigación (España)Sousa, J. Alejandro de [0000-0002-7948-8162]Damerio, Silvia [0000-0003-4460-9363]Koraltan, Sabri [0000-0002-1027-2232]Avci, Can Onur [0000-0003-1226-2342]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202520252025info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Publisher's versioninfo:eu-repo/semantics/publishedVersionhttp://hdl.handle.net/10261/385274https://api.elsevier.com/content/abstract/scopus_id/85216888579reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/MICINN/Plan Estatal de investigación Científica y Técnica y de Innovación 2021-2023/TED2021-129540A-I00info:eu-repo/grantAgreement/EC/H2020/949052info:eu-repo/grantAgreement/EC/HE/101106885info:eu-repo/grantAgreement/AEI/Plan Estatal de investigación Científica y Técnica y de Innovación 2021-2023/CEX2023-001263-SPhysical Review Appliedhttp://doi.org/10.1103/PhysRevApplied.23.014068Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3852742026-05-22T06:33:51Z
dc.title.none.fl_str_mv Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
title Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
spellingShingle Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
Sousa, J. Alejandro de
Metrology
Nernst effect
Spin Seebeck effect
Spin caloritronics
Transport phenomena
Heterostructures
Magnetic multilayers
Transition metals
title_short Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
title_full Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
title_fullStr Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
title_full_unstemmed Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
title_sort Decomposing measurements of the anomalous Nernst and spin Seebeck effects in Fe-based metallic multilayers
dc.creator.none.fl_str_mv Sousa, J. Alejandro de
Damerio, Silvia
Koraltan, Sabri
Avci, Can Onur
author Sousa, J. Alejandro de
author_facet Sousa, J. Alejandro de
Damerio, Silvia
Koraltan, Sabri
Avci, Can Onur
author_role author
author2 Damerio, Silvia
Koraltan, Sabri
Avci, Can Onur
author2_role author
author
author
dc.contributor.none.fl_str_mv Ministerio de Ciencia e Innovación (España)
European Commission
European Research Council
Agencia Estatal de Investigación (España)
Sousa, J. Alejandro de [0000-0002-7948-8162]
Damerio, Silvia [0000-0003-4460-9363]
Koraltan, Sabri [0000-0002-1027-2232]
Avci, Can Onur [0000-0003-1226-2342]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Metrology
Nernst effect
Spin Seebeck effect
Spin caloritronics
Transport phenomena
Heterostructures
Magnetic multilayers
Transition metals
topic Metrology
Nernst effect
Spin Seebeck effect
Spin caloritronics
Transport phenomena
Heterostructures
Magnetic multilayers
Transition metals
description Anomalous Nernst (ANE) and spin Seebeck effects (SSE) are ubiquitous in conducting magnetic materials subject to temperature gradients. Their characterization in metallic systems is especially strenuous because of their indistinguishable symmetry. Here, we report on the accurate characterization of the ANE and SSE in Fe-based multilayers at and above room temperature. We reveal that both effects consist of temperature-dependent and -independent components. At high temperatures, we provide evidence that the ANE decreases mainly due to reduced magnetization and spin polarization of free electrons, whereas the SSE increases owing to the enhanced thermal magnon density. We show that the relative strength of ANE and SSE can be tuned by thickness, stacking order, and doping concentration in various Fe-based multilayers, opening the way for thermoelectric device engineering.
publishDate 2025
dc.date.none.fl_str_mv 2025
2025
2025
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Publisher's version
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/385274
https://api.elsevier.com/content/abstract/scopus_id/85216888579
url http://hdl.handle.net/10261/385274
https://api.elsevier.com/content/abstract/scopus_id/85216888579
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv #PLACEHOLDER_PARENT_METADATA_VALUE#
#PLACEHOLDER_PARENT_METADATA_VALUE#
#PLACEHOLDER_PARENT_METADATA_VALUE#
#PLACEHOLDER_PARENT_METADATA_VALUE#
info:eu-repo/grantAgreement/MICINN/Plan Estatal de investigación Científica y Técnica y de Innovación 2021-2023/TED2021-129540A-I00
info:eu-repo/grantAgreement/EC/H2020/949052
info:eu-repo/grantAgreement/EC/HE/101106885
info:eu-repo/grantAgreement/AEI/Plan Estatal de investigación Científica y Técnica y de Innovación 2021-2023/CEX2023-001263-S
Physical Review Applied
http://doi.org/10.1103/PhysRevApplied.23.014068

dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869418093267124224
score 15,81155