Integrating 2D materials and plasmonics on lithium niobate platforms for pulsed laser operation at the nanoscale

The current need for coherent light sources for integrated (nano)photonics motivates the search for novel laser designs emitting at technologically relevant wavelengths with high-frequency stability and low power consumption. Here, a new monolithic architecture that integrates monolayer MoS2 and cha...

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Detalhes bibliográficos
Autores: Ramírez Herrero, María de la O, Molina de Pablo, Pablo, Hernández Pinilla, David, Lopez-Polin Peña, Guillermo, Ares García, Pablo, Lozano-Martín, Lidia, Yan, Han, Wang, Yan, Sarkar, Soumya, Al Shuhaib, Jinan H., Leardini, Fabrice, Gómez Herrero, Julio, Chhowalla, Manish, Bausa López, Luisa Eugenia
Formato: artículo
Fecha de publicación:2023
País:España
Recursos:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/709331
Acesso em linha:http://hdl.handle.net/10486/709331
https://dx.doi.org/10.1002/lpor.202300817
Access Level:acceso abierto
Palavra-chave:Lithium Niobate
2D Materials
Nanolasers
Plasmonic Chain
Rare earth emitters
Q-Switch
MoS 2
Física
Descrição
Resumo:The current need for coherent light sources for integrated (nano)photonics motivates the search for novel laser designs emitting at technologically relevant wavelengths with high-frequency stability and low power consumption. Here, a new monolithic architecture that integrates monolayer MoS2 and chains of silver nanoparticles on a rare-earth (Nd3+) doped LiNbO3 platform is developed to demonstrate Q-switched lasing operation at the nanoscale. The localized surface plasmons provided by the nanoparticle chains spatially confine the gain generated by Nd3+ ions at subwavelength scales, and large-area monolayer MoS2 acts as saturable absorber. As a result, an ultra-compact coherent pulsed light source delivering stable train pulses with repetition rates of hundreds of kHz and pulse duration of 1 µs is demonstrated without the need of any voltage-driven optical modulation. Moreover, the monolithic integration of the different elements is achieved without sophisticated processing, and it is compatible with LiNbO3-based photonics. The results highlight the robustness of the approach, which can be extended to other 2D materials and solid-state gain media. Potential applications in communications, quantum computing, or ultra-sensitive sensing can benefit from the synergy of the materials involved in this approach, which provides a wealth of opportunities for light control at reduced scales