Ionic circuitry with nanofluidic diodes

[EN] Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations...

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Detalles Bibliográficos
Autores: Ali, Mubarak, Nasir, Saima, Cervera, Javier, Mafe, Salvador, Ensinger, Wolfgang, Ramirez Hoyos, Patricio|||0000-0002-0067-4887
Tipo de recurso: artículo
Fecha de publicación:2019
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/214014
Acceso en línea:https://riunet.upv.es/handle/10251/214014
Access Level:acceso abierto
Palabra clave:Ionic circuits
Nanopores
Polyelectrolyte chains
Nanofluidic diodes
FISICA APLICADA
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spelling Ionic circuitry with nanofluidic diodesAli, MubarakNasir, SaimaCervera, JavierMafe, SalvadorEnsinger, WolfgangRamirez Hoyos, Patricio|||0000-0002-0067-4887Ionic circuitsNanoporesPolyelectrolyte chainsNanofluidic diodesFISICA APLICADA[EN] Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments.P. R., J. C., and S. M. acknowledge the funding from project PGC2018-097359-B-100, Spanish Ministry of Science and Education, and FEDER. M. A., S. N. and W. E. acknowledge the support from the LOEWE project iNAPO, Hessen State Ministry of Higher Education, Research and the Arts, Germany. The authors are thankful to Prof. C. Trautmann from GSI (Department of Material Research) for support with the heavy ion irradiation experiments and Mr E. Schubert for help in designing the electrochemical cells.The Royal Society of ChemistryDepartamento de Física AplicadaEscuela Técnica Superior de ArquitecturaCentro de Tecnologías Físicas: Acústica, Materiales y AstrofísicaAgencia Estatal de InvestigaciónEuropean Regional Development FundHessisches Ministerium für Wissenschaft und Kunst, AlemaniaRepositorio Institucional de la Universitat Politècnica de València Riunet20192019-12-21journal articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfapplication/pdfhttps://riunet.upv.es/handle/10251/214014reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valénciainstname:Universitat Politècnica de València (UPV)InglésengAgencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020 PGC2018-097359-B-I00 NANOESTRUCTURAS POROSAS DE INSPIRACION BIOLOGICA: ANALISIS Y CONTROL DE SEÑALES ELECTRICASopen accesshttp://purl.org/coar/access_right/c_abf2Reserva de todos los derechoshttp://rightsstatements.org/vocab/InC/1.0/info:eu-repo/semantics/openAccessoai:riunet.upv.es:10251/2140142026-06-13T07:49:27Z
dc.title.none.fl_str_mv Ionic circuitry with nanofluidic diodes
title Ionic circuitry with nanofluidic diodes
spellingShingle Ionic circuitry with nanofluidic diodes
Ali, Mubarak
Ionic circuits
Nanopores
Polyelectrolyte chains
Nanofluidic diodes
FISICA APLICADA
title_short Ionic circuitry with nanofluidic diodes
title_full Ionic circuitry with nanofluidic diodes
title_fullStr Ionic circuitry with nanofluidic diodes
title_full_unstemmed Ionic circuitry with nanofluidic diodes
title_sort Ionic circuitry with nanofluidic diodes
dc.creator.none.fl_str_mv Ali, Mubarak
Nasir, Saima
Cervera, Javier
Mafe, Salvador
Ensinger, Wolfgang
Ramirez Hoyos, Patricio|||0000-0002-0067-4887
author Ali, Mubarak
author_facet Ali, Mubarak
Nasir, Saima
Cervera, Javier
Mafe, Salvador
Ensinger, Wolfgang
Ramirez Hoyos, Patricio|||0000-0002-0067-4887
author_role author
author2 Nasir, Saima
Cervera, Javier
Mafe, Salvador
Ensinger, Wolfgang
Ramirez Hoyos, Patricio|||0000-0002-0067-4887
author2_role author
author
author
author
author
dc.contributor.none.fl_str_mv Departamento de Física Aplicada
Escuela Técnica Superior de Arquitectura
Centro de Tecnologías Físicas: Acústica, Materiales y Astrofísica
Agencia Estatal de Investigación
European Regional Development Fund
Hessisches Ministerium für Wissenschaft und Kunst, Alemania
Repositorio Institucional de la Universitat Politècnica de València Riunet
dc.subject.none.fl_str_mv Ionic circuits
Nanopores
Polyelectrolyte chains
Nanofluidic diodes
FISICA APLICADA
topic Ionic circuits
Nanopores
Polyelectrolyte chains
Nanofluidic diodes
FISICA APLICADA
description [EN] Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments.
publishDate 2019
dc.date.none.fl_str_mv 2019
2019-12-21
dc.type.none.fl_str_mv journal article
http://purl.org/coar/resource_type/c_6501
VoR
http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://riunet.upv.es/handle/10251/214014
url https://riunet.upv.es/handle/10251/214014
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.relation.none.fl_str_mv Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020 PGC2018-097359-B-I00 NANOESTRUCTURAS POROSAS DE INSPIRACION BIOLOGICA: ANALISIS Y CONTROL DE SEÑALES ELECTRICAS
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
Reserva de todos los derechos
http://rightsstatements.org/vocab/InC/1.0/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
Reserva de todos los derechos
http://rightsstatements.org/vocab/InC/1.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv The Royal Society of Chemistry
publisher.none.fl_str_mv The Royal Society of Chemistry
dc.source.none.fl_str_mv reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
instname:Universitat Politècnica de València (UPV)
instname_str Universitat Politècnica de València (UPV)
reponame_str RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
collection RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,811543

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