Visible-light mediated synthesis of bicalutamide by regioselective hydroxysulfonylation of acrylamides

Synthesis of anticancer drug bicalutamide promoted by visible light in one step from the corresponding N-arylacrylamide is described. This approach involves a one-pot hydroxysulfonylation reaction through a photocatalytic redox process. The use of Na2Eosin Y as photocatalyst and blue light allows th...

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Detalles Bibliográficos
Autores: Merino Marcos, Estibaliz|||0000-0002-2960-5404, Zurro de la Fuente, Mercedes|||0000-0003-1222-7926, Torres Oya, Sergio|||0000-0002-1003-519X
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universidad de Alcalá (UAH)
Repositorio:e_Buah Biblioteca Digital Universidad de Alcalá
Idioma:inglés
OAI Identifier:oai:ebuah.uah.es:10017/57892
Acceso en línea:http://hdl.handle.net/10017/57892
https://dx.doi.org/10.1002/ejoc.202300535
Access Level:acceso abierto
Palabra clave:Química
Chemistry
Descripción
Sumario:Synthesis of anticancer drug bicalutamide promoted by visible light in one step from the corresponding N-arylacrylamide is described. This approach involves a one-pot hydroxysulfonylation reaction through a photocatalytic redox process. The use of Na2Eosin Y as photocatalyst and blue light allows the access to a broad range of alfa-hydroxysulfonylamides bearing a quaternary center in moderate to good yields with complete regioselectivity via radical process.