Electrochemical fingerprint of archaeological lead silicate glasses from the voltammetry of microparticles approach

[EN] The application of a solid-state electrochemical technique, voltammetry of microparticles (VMP), for studying archeological lead glass is described. Upon attachment to graphite electrodes immersed into aqueous acetate buffer, characteristic voltammetric profiles were obtained for submicrosample...

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Detalles Bibliográficos
Autores: Doménech Carbó, Antonio, Villegas Broncano, María Ángeles, Martínez Ramírez, Sagrario, Martínez Pla, Betlem, Domenech Carbo, Mª Teresa|||0000-0003-3660-2161
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/151089
Acceso en línea:https://riunet.upv.es/handle/10251/151089
Access Level:acceso abierto
Palabra clave:Glass
Archaeometry
Voltammetry of microparticles
FIB-FESEM-EDX
Raman spectroscopy
PINTURA
Descripción
Sumario:[EN] The application of a solid-state electrochemical technique, voltammetry of microparticles (VMP), for studying archeological lead glass is described. Upon attachment to graphite electrodes immersed into aqueous acetate buffer, characteristic voltammetric profiles were obtained for submicrosamples of archeological glasses dated between the 9th and 19th centuries. Bivariate and multivariate chemometric analyses of the VMP data allowed us to characterize individual workshops/provenances which enabled a clear discrimination between soda-rich and potash-rich glasses. An analysis of the VMP data, combined by XRF, FESEM, AFM and ATR-FTIR and Micro-Raman spectroscopies, denoted the presence of Pb(IV) centers accompanying network-former and network-modifier Pb(II).