Heavy Mo isotope enrichment in the Pitcairn plume: Implications for the subduction cycle of anoxic sediments

Subduction redistributes elements between Earth's principal geochemical reservoirs, modifying the chemical composition of Earth's mantle, crust, atmosphere, and hydrosphere, and consequently having an impact on the evolution of life itself. Subduction of surface material that has been geoc...

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Detalhes bibliográficos
Autores: Ahmad, Qasid, Wille, Martin, Labidi, Jabrane, König, Stephan, Devey, Colin, Mezger, Klaus
Formato: artículo
Fecha de publicación:2023
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/344324
Acesso em linha:http://hdl.handle.net/10261/344324
Access Level:acceso abierto
Palavra-chave:Molybdenum isotopes
Enriched mantle
Pitcairn Island
LLSVP
Anoxic sediment
Subduction zones
Descrição
Resumo:Subduction redistributes elements between Earth's principal geochemical reservoirs, modifying the chemical composition of Earth's mantle, crust, atmosphere, and hydrosphere, and consequently having an impact on the evolution of life itself. Subduction of surface material that has been geochemically modified by low-temperature processes leads to mineralogical and chemical heterogeneities in mantle reservoirs over time and is recorded in modern ocean island basalts. One of the principal geochemical end members of the heterogeneous deep mantle, the enriched mantle 1 (EM-1) source of Pitcairn Island, has been attributed to the contribution of crustal material with vastly different chemical compositions and ages. The Mo isotope composition of lavas from Pitcairn Island constrains the nature of this recycled crustal component. Pitcairn lavas have elevated δMo relative to the depleted mantle. The high δMo is associated with high time-integrated Th/U and Rb/Sr, and low time-integrated Sm/Nd and U/Pb. These characteristics can be attributed to the recycling of nearly pristine pelagic sediments that were deposited in a Proterozoic anoxic deep-ocean into the sources of the Pitcairn Island lavas. The isotope composition of these lavas is similar to that of EM-1 hotspots from the South Atlantic, indicating the addition of reduced sediments in both of Earth's large low shear wave velocity provinces (LLSVPs). Consistent data from both locations imply that the subduction cycling of sedimentary redox-sensitive elements such as Mo, S, Se, and U into arc magmas was in these cases inefficient in the Precambrian and the chemical and isotopic signature of reduced sediments is preserved in the source of ocean island basalts bearing the EM-1 characteristics.