Molybdenum isotopes in plume-influenced MORBs reveal recycling of ancient anoxic sediments

Under modern oxidising Earth surface conditions, dehydrated subducted slabs show Mo isotope compositions as low as δMo = −1.5 %, compared to the depleted mantle δMo = −0.2 %. Such light Mo isotope compositions reflect the redox-dependent aqueous mobility of isotopically heavy Mo associated with slab...

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Detalhes bibliográficos
Autores: Ahmad, Qasid, Wille, M., Rosca, Carolina, Labidi, J., Schmid, T., Mezger, Klaus, König, Stephan
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2022
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositório:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/357196
Acesso em linha:http://hdl.handle.net/10261/357196
Access Level:Acceso aberto
Palavra-chave:Atlantic Ocean
Mid-Atlantic Ridge
Anoxic conditions
Glass
Isotopic composition
Isotopic fractionation
Molybdenum
Plume
Proterozoic
Sedimentation
Subduction
Descrição
Resumo:Under modern oxidising Earth surface conditions, dehydrated subducted slabs show Mo isotope compositions as low as δMo = −1.5 %, compared to the depleted mantle δMo = −0.2 %. Such light Mo isotope compositions reflect the redox-dependent aqueous mobility of isotopically heavy Mo associated with slab dehydration. Here we analysed basaltic glasses from the South-Mid Atlantic Ridge, whose parental melts are influenced by the enriched Discovery and Shona mantle plumes. We report increasingly higher δMo of up to −0.1 % from the most depleted samples towards those tapping more enriched mantle sources. δMo values correlate with radiogenic Sr and Nd isotopes, which indicates the recycling of Proterozoic sediments with a Mo isotopic composition that was not affected by subduction-related, oxic dehydration. We propose that the Mo isotope signatures were retained during subduction and reflect anoxic conditions during deep sea sedimentation in the mid-Proterozoic. Finally, Mo isotope fractionation between different terrestrial reservoirs likely depends on the slab redox budget, and therefore on the timing of subduction with regard to Earth’s surface oxygenation.