He4 Adsorbed on the Outer Surface of Carbon Nanotube Bundles

The results of diffusion Monte Carlo calculations on the behavior of He4 adsorbed on the external surface of a bundle of carbon nanotubes are presented. The corrugation effects are found to be very important, making the outside part of the bundles a quite inhomogeneous substrate. No stable solid hel...

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Detalles Bibliográficos
Autor: Gordillo, M.C.
Tipo de recurso: artículo
Fecha de publicación:2008
País:España
Institución:Universidad Pablo de Olavide (UPO)
Repositorio:RIO. Repositorio Institucional Olavide
Idioma:inglés
OAI Identifier:oai:rio.upo.es:10433/934
Acceso en línea:http://hdl.handle.net/10433/934
Access Level:acceso abierto
Palabra clave:Monte Carlo calculations
Carbon nanotubes
Descripción
Sumario:The results of diffusion Monte Carlo calculations on the behavior of He4 adsorbed on the external surface of a bundle of carbon nanotubes are presented. The corrugation effects are found to be very important, making the outside part of the bundles a quite inhomogeneous substrate. No stable solid helium monolayer at high density was found. Instead, helium atoms are promoted to a second quasi-one-dimensional phase on top of the liquid first layer. On increasing the helium intake, a two layer structure is formed in which the helium directly in contact with the carbon surface solidifies.