Electrochemical Tuning of Metal Insulator Transition and Nonvolatile Resistive Switching in Superconducting Films

Modulation of carrier concentration in strongly correlated oxides offers the unique opportunity to induce different phases in the same material, which dramatically change their physical properties, providing novel concepts in oxide electronic devices with engineered functionalities. This work report...

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Detalles Bibliográficos
Autores: Palau, Anna, Fernández Rodríguez, Alejandro, Gonzalez Rosillo, Juan Carlos, Granados, Xavier, Coll, Mariona, Bozzo, Bernat, Ortega Hernandez, Rafael, Suñé, Jordi, Mestres, Narcís, Obradors, Xavier, Puig Molina, Teresa
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2018
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/173969
Acceso en línea:http://hdl.handle.net/10261/173969
Access Level:acceso abierto
Palabra clave:Electrochemical oxygen doping
Strongly correlated oxides
Metal-insulator transitions
Reversible switching
High temperature superconductors
Descripción
Sumario:Modulation of carrier concentration in strongly correlated oxides offers the unique opportunity to induce different phases in the same material, which dramatically change their physical properties, providing novel concepts in oxide electronic devices with engineered functionalities. This work reports on the electric manipulation of the superconducting to insulator phase transition in YBa2Cu3O7−δ thin films by electrochemical oxygen doping. Both normal state resistance and the superconducting critical temperature can be reversibly manipulated in confined active volumes of the film by gate-tunable oxygen diffusion. Vertical and lateral oxygen mobility may be finely modulated, at the micro- and nano-scale, by tuning the applied bias voltage and operating temperature thus providing the basis for the design of homogeneous and flexible transistor-like devices with loss-less superconducting drain–source channels. We analyze the experimental results in light of a theoretical model, which incorporates thermally activated and electrically driven volume oxygen diffusion.