Shaping Techniques' Influence on the Electrochemical Properties of BaCe0.6Zr0.3Y0.1O3-δ proton conductor

Hydrogen's significance as a clean and high-energy source spans various industries, driving advancements in fuel cell technology, transportation, and renewable energy storage systems. In particular, solid-state proton conductors like perovskite-type materials exhibit promising attributes for ap...

Full description

Bibliographic Details
Authors: Hinojo, Antonio, Lujan, Enric, Verdaguer, Ariadna, Abella, Jordi, Colominas, Sergi
Format: article
Publication Date:2024
Country:España
Institution:Universitat Ramon Llull (URL)
Repository:DAU Arxiu Digital de la Universitat Ramon Llull
OAI Identifier:oai:dau.url.edu:20.500.14342/5308
Online Access:http://hdl.handle.net/20.500.14342/5308
https://doi.org/10.1016/j.ceramint.2024.05.447
Access Level:Embargoed access
Keyword:BCZY
Proton conductivity
Shaping
3D printing
CIP
Perovskites
Conductor protònic
Impressió 3D
Perovskita
54
620
Description
Summary:Hydrogen's significance as a clean and high-energy source spans various industries, driving advancements in fuel cell technology, transportation, and renewable energy storage systems. In particular, solid-state proton conductors like perovskite-type materials exhibit promising attributes for applications such as fuel cells and hydrogen sensors. However, conventional shaping techniques like uniaxial pressing impose limitations on device scalability and geometry. To address these challenges, alternative methods are gaining traction, like cold isostatic pressing or additive manufacturing. Each technique offers distinct advantages in shaping materials, impacting their structural and morphological properties. In this study, pellets of BaCe0.6Zr0.3Y0.1O3-δ (BCZY) solid-state electrolyte were fabricated using four different shaping techniques: uniaxial pressing, cold isostatic pressing, 3D extrusion, and lithography. Characterization via X-ray diffraction, scanning electron microscopy, and electrochemical impedance spectroscopy provided insights into changes in crystalline structure, sintering quality, and electrochemical properties, respectively.