Giant spin lifetime anisotropy in graphene induced by proximity effects

We report on fundamental aspects of spin dynamics in heterostructures of graphene and transition metal dichalcogenides (TMDCs). By using realistic models derived from first principles we compute the spin lifetime anisotropy, defined as the ratio of lifetimes for spins pointing out of the graphene pl...

Descripción completa

Detalles Bibliográficos
Autores: Cummings, Aron|||0000-0003-2307-497X, Garcia, José H.|||0000-0002-5752-4759, Fabian, Jaroslav|||0000-0002-3009-4525, Roche, Stephan|||0000-0003-0323-4665
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:194891
Acceso en línea:https://ddd.uab.cat/record/194891
https://dx.doi.org/urn:doi:10.1103/PhysRevLett.119.206601
Access Level:acceso abierto
Palabra clave:First principles
Proximity effects
Realistic model
Spin degrees of freedom
Spin relaxation
Spin-orbit couplings
Spintronic device
Transition metal dichalcogenides
Descripción
Sumario:We report on fundamental aspects of spin dynamics in heterostructures of graphene and transition metal dichalcogenides (TMDCs). By using realistic models derived from first principles we compute the spin lifetime anisotropy, defined as the ratio of lifetimes for spins pointing out of the graphene plane to those pointing in the plane. We find that the anisotropy can reach values of tens to hundreds, which is unprecedented for typical 2D systems with spin-orbit coupling and indicates a qualitatively new regime of spin relaxation. This behavior is mediated by spin-valley locking, which is strongly imprinted onto graphene by TMDCs. Our results indicate that this giant spin lifetime anisotropy can serve as an experimental signature of materials with strong spin-valley locking, including graphene-TMDC heterostructures and TMDCs themselves. Additionally, materials with giant spin lifetime anisotropy can provide an exciting platform for manipulating the valley and spin degrees of freedom, and for designing novel spintronic devices.