Room-temperature spin hall effect in graphene/MoS2 van der Waals heterostructures

Graphene is an excellent material for long-distance spin transport but allows little spin manipulation. Transition-metal dichalcogenides imprint their strong spin-orbit coupling into graphene via the proximity effect, and it has been predicted that efficient spin-to-charge conversion due to spin Hal...

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Bibliographic Details
Authors: Safeer, Chenattukuzhiyil, Ingla-Aynés, Josep, Herling, Franz, Garcia, José H.|||0000-0002-5752-4759, Vila Tusell, Marc|||0000-0001-9118-421X, Ontoso, Nerea, Calvo, M. Reyes, Roche, Stephan|||0000-0003-0323-4665, Hueso, Luis E., Casanova, Fèlix
Format: article
Publication Date:2019
Country:España
Institution:Universitat Autònoma de Barcelona
Repository:Dipòsit Digital de Documents de la UAB
Language:English
OAI Identifier:oai:ddd.uab.cat:211669
Online Access:https://ddd.uab.cat/record/211669
https://dx.doi.org/urn:doi:10.1021/acs.nanolett.8b04368
Access Level:Open access
Keyword:Graphene
Transition metal dichalcogenides
Spintronics
Spin Hall effect
Rashba-Edelstein effect
Description
Summary:Graphene is an excellent material for long-distance spin transport but allows little spin manipulation. Transition-metal dichalcogenides imprint their strong spin-orbit coupling into graphene via the proximity effect, and it has been predicted that efficient spin-to-charge conversion due to spin Hall and Rashba-Edelstein effects could be achieved. Here, by combining Hall probes with ferromagnetic electrodes, we unambiguously demonstrate experimentally the spin Hall effect in graphene induced by MoS proximity and for varying temperatures up to room temperature. The fact that spin transport and the spin Hall effect occur in different parts of the same material gives rise to a hitherto unreported efficiency for the spin-to-charge voltage output. Additionally, for a single graphene/MoS heterostructure-based device, we evidence a superimposed spin-to-charge current conversion that can be indistinguishably associated with either the proximity-induced Rashba-Edelstein effect in graphene or the spin Hall effect in MoS. By a comparison of our results to theoretical calculations, the latter scenario is found to be the most plausible one. Our findings pave the way toward the combination of spin information transport and spin-to-charge conversion in two-dimensional materials, opening exciting opportunities in a variety of future spintronic applications.