Recent advances on asymmetric nitroso aldol reaction

The reaction of aromatic nitroso derivatives with enolizable carbonyl compounds (nitroso aldol reaction) to give either α-hydroxyamino or α-aminoxy carbonyl compounds is an important synthetic method. This review illustrates the recent advances in rendering the process regio- and enantioselective as...

Descripción completa

Detalles Bibliográficos
Autores: Merino, Pedro, Tejero, Tomás, Delso, J. Ignacio, Matute, Rosa
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2016
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/155774
Acceso en línea:http://hdl.handle.net/10261/155774
Access Level:acceso abierto
Palabra clave:Aminoxylation
Asymmetric nitroso aldol
α-amino carbonyls
Hydroxyamination
Organocatalysts
α-hydroxy carbonyls
Descripción
Sumario:The reaction of aromatic nitroso derivatives with enolizable carbonyl compounds (nitroso aldol reaction) to give either α-hydroxyamino or α-aminoxy carbonyl compounds is an important synthetic method. This review illustrates the recent advances in rendering the process regio- and enantioselective as well as catalytic. By employing metal and organic catalysts a range of α-amino (α-oxyamination) and α-hydroxy (α-aminoxylation) carbonyl derivatives can be generated with total regioselectivity and high levels of enantiomeric excess.