Synthesis and reactivity of di(silylamido)cyclopentadienyl titanium and zirconium complexes

We present in this account the synthesis and recent developments of a new class of group 4 metal complexes with the tridentate di(silylamido)cyclopentadienyl ligand. These doubly silyl-bridged group 4 metal amido chelates are receiving increasing interest as they are efficient catalysts for ethene p...

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Detalles Bibliográficos
Autores: Cano Sierra, Jesús|||0000-0002-6643-7534, Sudupe Ormeño, María, Royo Gracia, Pascual
Tipo de recurso: artículo
Fecha de publicación:2007
País:España
Institución:Universidad de Alcalá (UAH)
Repositorio:e_Buah Biblioteca Digital Universidad de Alcalá
Idioma:inglés
OAI Identifier:oai:ebuah.uah.es:10017/4170
Acceso en línea:http://hdl.handle.net/10017/4170
https://dx.doi.org/10.1016/j.jorganchem.2007.06.049
Access Level:acceso abierto
Palabra clave:Silylamido
Cyclopentadienyl
Titanium
Zirconium
Ciencia
Química inorgánica
Chemistry, inorganic
Science
Descripción
Sumario:We present in this account the synthesis and recent developments of a new class of group 4 metal complexes with the tridentate di(silylamido)cyclopentadienyl ligand. These doubly silyl-bridged group 4 metal amido chelates are receiving increasing interest as they are efficient catalysts for ethene polymerization when activated with MAO despite generating 14-electron d0 cationic species free of the alkyl group required for the first insertion reaction in the polymerization process.