Transient scattering effects and electron plasma dynamics during ultrafast laser ablation of water

We study the dynamics of single-shot ultrafast laser ablation of a water-gas interface. We model the extremely nonlinear light-water interaction during the first picosecond by simulating the laser pulse propagation while dynamically calculating the spatial distribution of the dielectric function. We...

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Bibliographic Details
Authors: Hernández Rueda, Francisco Javier, Van Oosten, Dries
Format: article
Publication Date:2019
Country:España
Institution:Universidad Complutense de Madrid (UCM)
Repository:Docta Complutense
Language:English
OAI Identifier:oai:docta.ucm.es:20.500.14352/105014
Online Access:https://hdl.handle.net/20.500.14352/105014
Access Level:Open access
Keyword:535
Induced shockwaves
Breakdown
Waves
Air
Óptica (Física)
2209 Óptica
Description
Summary:We study the dynamics of single-shot ultrafast laser ablation of a water-gas interface. We model the extremely nonlinear light-water interaction during the first picosecond by simulating the laser pulse propagation while dynamically calculating the spatial distribution of the dielectric function. We make use of a finite-difference time-domain algorithm to solve Maxwell's equations and Rethfeld's multiple rate equation model to consider the local excitation of a dense electron plasma. We validate our model by comparing the simulated transient reflectivity with experimental results and find excellent agreement. (C) 2019 Optical Society of America