Slowing-down of non-equilibrium concentration fluctuations in confinement

Fluctuations in a fluid are strongly affected by the presence of a macroscopic gradient making them long- ranged and enhancing their amplitude. While small-scale fluctuations exhibit diffusive lifetimes, moderate-scale fluctuations live shorter because of gravity. In this letter we explore fluctuati...

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Detalles Bibliográficos
Autores: Giraudet, Cédric, Bataller, Henri, Sun, Yifei, Donev, Aleksander, Ortiz De Zárate Leira, José María, Croccolo, Fabrizio
Tipo de recurso: artículo
Fecha de publicación:2015
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/24282
Acceso en línea:https://hdl.handle.net/20.500.14352/24282
Access Level:acceso abierto
Palabra clave:536
Liquid-mixtures
Free diffusion
Gravity
Fluids
Soret
Microgravity
Shadowgraph
Scattering
Schlieren
Termodinámica
2213 Termodinámica
Descripción
Sumario:Fluctuations in a fluid are strongly affected by the presence of a macroscopic gradient making them long- ranged and enhancing their amplitude. While small-scale fluctuations exhibit diffusive lifetimes, moderate-scale fluctuations live shorter because of gravity. In this letter we explore fluctuations of even larger size, comparable to the extent of the system in the direction of the gradient, and find experimental evidence of a dramatic slowing-down of their dynamics. We recover diffusive behavior for these strongly confined fluctuations, but with a diffusion coefficient that depends on the solutal Rayleigh number. Results from dynamic shadowgraph experiments are complemented by theoretical calculations and numerical simulations based on fluctuating hydrodynamics, and excellent agreement is found. Hence, the study of the dynamics of non-equilibrium fluctuations allows to probe and measure the competition of physical processes such as diffusion, buoyancy and confinement, i.e. the ingredients included in the Rayleigh number, which is the control parameter of our system.