Confinement effect on the dynamics of non-equilibrium concentration fluctuations far from the onset of convection

In a recent letter (C. Giraudet et al., EPL 111, 60013 (2015)) we reported preliminary data showing evidence of a slowing-down of non-equilibrium fluctuations of the concentration in thermodiffusion experiments on a binary mixture of miscible fluids. The reason for this slowing-down was attributed t...

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Detalhes bibliográficos
Autores: Giraudet, Cédric, Bataller, Henri, Sun, Yifei, Donev, Aleksandar, Ortiz De Zárate Leira, José María, Croccolo, Fabrizio
Tipo de documento: artigo
Data de publicação:2016
País:España
Recursos:Universidad Complutense de Madrid (UCM)
Repositório:Docta Complutense
Idioma:inglês
OAI Identifier:oai:docta.ucm.es:20.500.14352/17710
Acesso em linha:https://hdl.handle.net/20.500.14352/17710
Access Level:Acceso aberto
Palavra-chave:536
Mass-transport properties
Liquid-mixtures
Free-diffusion
Thermal-diffusion
Light-scattering
Soret
Gravity
Equilibrium
Fluid
Microgravity
Termodinámica
2213 Termodinámica
Descrição
Resumo:In a recent letter (C. Giraudet et al., EPL 111, 60013 (2015)) we reported preliminary data showing evidence of a slowing-down of non-equilibrium fluctuations of the concentration in thermodiffusion experiments on a binary mixture of miscible fluids. The reason for this slowing-down was attributed to the effect of confinement. Such tentative explanation is here experimentally corroborated by new measurements and theoretically substantiated by studying analytically and numerically the relevant fluctuating hydrodynamics equations. In the new experiments presented here, the magnitude of the temperature gradient is changed, confirming that the system is controlled solely by the solutal Rayleigh number, and that the slowing-down is dominated by a combined effect of the driving force of buoyancy, the dissipating force of diffusion and the confinement provided by the vertical extension of the sample cell. Moreover, a compact phenomenological interpolating formula is proposed for easy analysis of experimental results.