Electroinduced crosslinking of triphenylamine-based polybenzoxazines

Polybenzoxazines attract much attention as good phenolic resins due to their interesting and useful properties. Recently, benzoxazine monomers have been employed as crosslinking agents to enhance the properties of different types of polymers by being used as additives to a secondary cure process. In...

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Detalles Bibliográficos
Autores: Gascó-Catalán, Carolina|||0000-0003-4435-8306, Rodríguez-Santiago, Luis|||0000-0003-4983-4228, Sodupe, Mariona|||0000-0003-0276-0524, Sebastián, Rosa María|||0000-0001-5519-9131, Guirado, Gonzalo|||0000-0003-2128-7007
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:265731
Acceso en línea:https://ddd.uab.cat/record/265731
https://dx.doi.org/urn:doi:10.1016/j.microc.2022.107878
Access Level:acceso abierto
Palabra clave:Polybenzoxazines
Electrochemistry
Electroinduced crosslinking
Descripción
Sumario:Polybenzoxazines attract much attention as good phenolic resins due to their interesting and useful properties. Recently, benzoxazine monomers have been employed as crosslinking agents to enhance the properties of different types of polymers by being used as additives to a secondary cure process. In this paper, we propose a new electroinduced approach to increase the crosslinking density of electroactive polybenzoxazines through the design of new monomers that contain triphenylamine groups as electrodimerization points. The use of electrochemical techniques means the crosslinking process can be monitored and also the electrochemical reaction process upon polybenzoxazine oxidation either in solution or ionogel matrixes can be disclosed. These studies lay the foundations for the design of smart polybenzoxazines that could undergo dual-cure mechanisms at low electrochemical potential values.