Enhanced CO2 affinity in a metal-organic framework through green incorporation of a dual-functional amino acid

Post-synthetic incorporation of amino acids into the Zr-based metal-organic framework DUT-67 via relatively green methods yields materials with enhanced CO2 affinity. Structural and sorption studies reveal high affinity for DUT-67-Trp, exploiting its dual functionality to achieve an adsorption entha...

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Detalles Bibliográficos
Autores: Loukopoulos, Edward, Barragán-Soto, Sofía, Marugán-Benito, Sergio, Borrego-Marin, Emilio, Navarro, Jorge A R, Platero-Prats, Ana E.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2025
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/422065
Acceso en línea:http://hdl.handle.net/10261/422065
https://api.elsevier.com/content/abstract/scopus_id/105027525329
Access Level:acceso abierto
Descripción
Sumario:Post-synthetic incorporation of amino acids into the Zr-based metal-organic framework DUT-67 via relatively green methods yields materials with enhanced CO2 affinity. Structural and sorption studies reveal high affinity for DUT-67-Trp, exploiting its dual functionality to achieve an adsorption enthalpy level comparable to those of high-performing frameworks. The findings provide a promising pathway towards developing sustainable amino-functionalized CO2 sorbents.