Organocatalytic Enantioselective Strecker Reaction with Seven-Membered Cyclic Imines

[EN] A highly enantioselective Strecker reaction with dibenzo[b,f][1,4]oxazepines has been described using a dihydroquinine-derived thiourea as organocatalyst. The reaction affords chiral 10,11-dihydrodibenzo[b,f][1,4] oxazepine 11-carbonitrile derivatives in excellent yields (up to 99%) and excelle...

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Detalles Bibliográficos
Autores: Lluna Galán, C., Blay, G., Fernández, I., Pedro, J. R., Vila, C., Muñoz Roca, María Del Carmen|||0000-0003-2630-3897
Tipo de recurso: artículo
Fecha de publicación:2018
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/132857
Acceso en línea:https://riunet.upv.es/handle/10251/132857
Access Level:acceso abierto
Palabra clave:Asymmetric catalysis
Organocatalysis
Strecker reaction
Dibenzo[b,f][1,4]oxazepines
Alpha-amino nitriles
FISICA APLICADA
Descripción
Sumario:[EN] A highly enantioselective Strecker reaction with dibenzo[b,f][1,4]oxazepines has been described using a dihydroquinine-derived thiourea as organocatalyst. The reaction affords chiral 10,11-dihydrodibenzo[b,f][1,4] oxazepine 11-carbonitrile derivatives in excellent yields (up to 99%) and excellent enantioselectivities (up to 98%) under mild reaction conditions.