Regiodivergent Deuteration of Pyridine-Based Heterocycles

Herein, we describe a regiodivergent deuteration of pyridotriazoles under mild conditions. Site-selective deuteration can be tuned, controlled, and switched by a subtle interplay of the base and solvent utilized. Given the ease at which pyridotriazoles can be converted into a variety of pyridine con...

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Detalhes bibliográficos
Autores: Du, Wei, Gadekar, Santosh C., Velasco-Rubio, Álvaro, Rodrigalvarez, Jesus, Martin, Ruben
Formato: artículo
Fecha de publicación:2025
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/487540
Acesso em linha:http://hdl.handle.net/2072/487540
https://doi.org/10.1021/acs.orglett.5c02961
Access Level:acceso abierto
Palavra-chave:Química
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Descrição
Resumo:Herein, we describe a regiodivergent deuteration of pyridotriazoles under mild conditions. Site-selective deuteration can be tuned, controlled, and switched by a subtle interplay of the base and solvent utilized. Given the ease at which pyridotriazoles can be converted into a variety of pyridine congeners, this protocol might offer a new gateway to access a variety of deuterium-labeled pyridine-containing heterocycles in a site-selective, yet predictable, manner.